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Record W4385285184 · doi:10.1021/acsomega.3c03178

Simultaneous Determination of 147 Pesticide Residues in Traditional Chinese Medicines by GC–MS/MS

2023· article· en· W4385285184 on OpenAlexafffund
Chao Ji, Xingyu Wang, Marti Z. Hua, Yifeng Wu, Yifan Wang, Zhiqiang Wu, Xiahong He, Dunming Xu, Wenjie Zheng, Xiaonan Lu

Bibliographic record

VenueACS Omega · 2023
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicPesticide Residue Analysis and Safety
Canadian institutionsMcGill University
FundersNational Key Research and Development Program of ChinaEarmarked Fund for China Agriculture Research SystemKunming Science and Technology BureauMcGill University
KeywordsQuechersChromatographyPesticideChemistryGas Chromatography/Tandem Mass SpectrometryPesticide residueGas chromatography–mass spectrometrySolid phase extractionExtraction (chemistry)Ethyl acetateTandem mass spectrometryMass spectrometryHoneysuckle

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Determination of pesticide residues remains a challenge in traditional Chinese medicines in which complex compounds may interfere with analysis signals. This study reports the development of a simple, effective, and high-throughput method combining gas chromatography–tandem mass spectrometry (GC–MS/MS) with either QuEChERS or solid phase extraction (SPE) to determine 147 pesticide residues in traditional Chinese medicines simultaneously. In SPE, the mixture of n -hexane and ethyl acetate (1:1, v/v) was selected to extract 147 pesticides in honeysuckle, and the extracted pesticides were determined by GC–MS/MS. The limits of detection for all pesticides were within 0.01–0.05 mg/kg. The recoveries were within 70–120% and the relative standard deviations were below 20% for over 90% pesticides. The coefficients of determination were up to 0.999 for the linearity between MS signals and different concentrations of pesticides (20–200 ng/mL). The analytical performance was confirmed in determining pesticide residues in dried tangerine peel. SPE achieved comparable recoveries for all pesticides compared to the QuEChERS method.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.253
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueACS OmegaSame topicPesticide Residue Analysis and SafetyFrench-language works237,207