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Record W4385382944 · doi:10.3749/2200051

Cation Ordering in Spinel from Calcium-Aluminum-Rich Inclusions in Carbonaceous Chondrites NWA 2364 and NWA 6991 to Quantify Temperature in the Early Solar System

2023· article· en· W4385382944 on OpenAlexaff
Victoria L. Houde, R. L. Flemming, Audrey Bouvier, Victor V. Terskikh

Bibliographic record

VenueThe Canadian Journal of Mineralogy and Petrology · 2023
Typearticle
Languageen
FieldChemistry
TopicAdvanced NMR Techniques and Applications
Canadian institutionsNational Research Council CanadaWestern University
Fundersnot available
KeywordsSpinelChondriteDiopsideMagic angle spinningMineralMaterials scienceAnalytical Chemistry (journal)MineralogyMeteoriteChemistryNuclear magnetic resonance spectroscopyPhysics

Abstract

fetched live from OpenAlex

Abstract Minerals extracted from two calcium-aluminum-rich inclusions, one each from NWA 2364 and NWA 6991 CV3 chondrite meteorites, were examined using micro X-ray diffraction, 27Al magic angle spinning nuclear magnetic resonance spectroscopy (MAS NMR) and Triple Quantum (3Q) MAS NMR. In situ examination by micro X-ray diffraction was used to confirm the presence of spinel (MgAl2O4) and to identify co-existing minerals. Aluminum-27 3Q MAS NMR was used to confirm the identity of co-existing minerals by their NMR signature in this two-dimensional experiment and to ensure that their NMR peaks did not overlap with those attributed to spinel. Aluminum-27 MAS NMR was used to quantitatively measure cation ordering between the tetrahedral ([4]Al) and octahedral ([6]Al) sites in the spinel. The measured cation distribution was used to calculate the inversion parameter, x, for each sample: x = 0.077 ± 0.007 for NWA 2364, x = 0.027 ± 0.001 for NWA 6991 (gehlenite-rich fraction), and x = 0.052 ± 0.003 for NWA 6991 (Al-bearing diopside-rich fraction). The measured cation-ordering data were input into six literature calibration curves to estimate the temperature of formation or the most recent equilibration temperature of the spinel. The NWA 2364 sample yielded temperatures between 420 and 707 K and the NWA 6991 sample yielded temperatures between 153 and 615 K, depending on the calibration curve used. These temperatures are lower than expected for nebular condensation temperatures, however, reordering may have occurred during cooling from high temperatures, so these values may be taken to represent temperature minima. The calculated spinel-related temperatures may thus represent equilibration temperatures related to subsequent nebular or CV chondrite parent body processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.019

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.266
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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