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Record W4386639869 · doi:10.26434/chemrxiv-2023-kzgfb

Spy1-activated Cyclin Dependent Kinase 2 Shows Reduced Affinity for Current Synthetic Small Molecule Inhibitors of the CDK2-Cyclin Complex

2023· preprint· en· W4386639869 on OpenAlexafffund
Daniel Meister, John J. Hayward, Bre‐Anne Fifield, Lisa A. Porter, John F. Trant

Bibliographic record

VenueChemRxiv · 2023
Typepreprint
Languageen
FieldMedicine
TopicAdvanced Breast Cancer Therapies
Canadian institutionsUniversity of Windsor
FundersNatural Sciences and Engineering Research Council of CanadaCanadian Institutes of Health ResearchAlliance de recherche numérique du CanadaOntario Institute for Cancer Research
KeywordsCyclin-dependent kinaseCyclin-dependent kinase 2CyclinSmall moleculeBiologyKinaseCyclin ACDK inhibitorCancer researchCell cycleCell biologyProtein kinase ABiochemistryCell

Abstract

fetched live from OpenAlex

Cyclin-dependent kinases (CDKs) play a key role in activating essential cell biology processes including cellular proliferation. Inappropriate regulation of CDKs has been implicated in driving several different forms of cancer. One of the regulatory factors is the need to bind to Cyclin-partners before they can be activated and advance the cell cycle. Cyclins are overexpressed in several different cancers, hence activating their relevant CDK. Hyperactive CDK2 in particular is implicated in many cancers, and while many drugs have shown preclinical promise, none have successfully passed through clinical development. Among the complications of targeting CDK2 is the fact that non-classical cyclin partners from the Speedy/RINGO family of proteins can alter the conformation of the kinase. Using computational approaches, we provide data supporting that the active site of CDK2 differs when bound to Spy1 as compared to classical cyclins. Furthermore, combining computational models with experimental techniques we provide data that many small molecule inhibitors have reduced activity against Spy1-bound CDKs. This work supports the need to develop new inhibitors capable of inhibiting the Spy1-CDK2 complex, and suggests that computational tools can be beneficial toward accomplishing this goal.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.026
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.099
GPT teacher head0.339
Teacher spread0.239 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2023
Admission routes2
Has abstractyes

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