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Record W4386640758 · doi:10.1002/elan.202300072

Simultaneous detection of trace Pb(II) and Cd(II) cations in ore samples by anodic stripping analysis using pMO/erGO‐modified glassy carbon electrodes

2023· article· en· W4386640758 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueElectroanalysis · 2023
Typearticle
Languageen
FieldChemistry
TopicElectrochemical Analysis and Applications
Canadian institutionsUniversité du Québec à Chicoutimi
FundersDivision of Chemistry
KeywordsDetection limitAnodic stripping voltammetryElectrodeAnalytical Chemistry (journal)GrapheneStripping (fiber)Materials scienceElectrochemistryMetal ions in aqueous solutionRaman spectroscopyGlassy carbonChemistryInorganic chemistryCyclic voltammetryMetalNanotechnologyChromatographyMetallurgy

Abstract

fetched live from OpenAlex

Abstract Environmental safety is of paramount importance for human well‐being, imposing significant demands for affordable, rapid, portable, and robust analytical tools for real‐time and on‐site water monitoring. In this context, we have developed an analytical method to efficiently detect heavy metal ions, particularly Pb 2+ ions, in water samples. This method employs a stepwise‐prepared electrode comprised of a thin film of poly(methyl orange) (pMO) electrochemically deposited onto reduced graphene oxide (erGO), which is in turn coated on a glassy carbon electrode (GCE). The resulting pMO/erGO/GCE electrode was characterized using Raman spectroscopy, scanning electron microscopy (SEM), and electrochemical techniques. Square wave anodic stripping voltammetry (SWASV) was subsequently employed to detect the target ions. Importantly, the pMO/erGO/GCE electrode exhibits excellent analytical performance, featuring a broad linear concentration range spanning from 14 to 595 parts per billion (ppb), a sensitivity of 5.60 μA ppb −1 cm −2 , and a theoretical calculated value of the detection limit of 0.82 ppb. The effectiveness of this sensor was validated through successful testing of aqueous samples from dissolved ores containing both lead(II) and cadmium(II) cations, as determined by atomic absorption spectroscopy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.300
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.010
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.247
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it