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Record W4386867021 · doi:10.1149/ma2023-0172850mtgabs

Investigation of Reduced Graphene Oxide Modified Zinc Anodes Using Various Electrochemical Techniques

2023· article· en· W4386867021 on OpenAlexaff
Andrew Sellathurai, Dominik P. J. Barz, Bo Xiao Zhang

Bibliographic record

VenueECS Meeting Abstracts · 2023
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsQueen's University
Fundersnot available
KeywordsGrapheneAnodeZincElectrolyteOverpotentialSeparator (oil production)Materials sciencePassivationChemical engineeringNucleationElectrochemistryOxideCoatingInorganic chemistryElectrodeChemistryNanotechnologyMetallurgyOrganic chemistry

Abstract

fetched live from OpenAlex

Zinc ion batteries are promising battery energy storage systems due to their high capacity, abundancy and low cost, but are held back by competing reactions, passivation, and dendrite formation which all greatly reduce performance. We modify zinc anode by introducing a self-reducing graphene oxide coating. This protects against dendrite formation and reduces side reactions, increasing the performance of the cell. Half-cell experiments are performed to determine whether sodium sulphate, sodium acetate, or a combination of the provides any advantage over the other, as well as to determine the effect the pattern of the reduced graphene oxide coating on performance. Additionally, symmetric zinc coin cells are assembled, and studied by galvanostatic charge/discharge cycles, and chronopotentiometry. The effect of the reduced graphene oxide coating, electrolyte composition, choice of separator (paper/glass) on the cycling stability and over potential of zinc deposition is studied. The partially covered (island) zinc anode greatly reduces the nucleation overpotential to 8.75 mV when assembled in a symmetric coin cell. Excellent cycling stability is observed at a current density of 5 mA cm -2 charged to 5 mAh cm -2 when using a combination background electrolyte of sodium sulphate and sodium acetate using a glass fibre separator.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.058
Threshold uncertainty score0.781

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.034
GPT teacher head0.280
Teacher spread0.245 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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