MétaCan
Menu
Back to cohort
Record W4388680724 · doi:10.1002/maco.202314054

Temperature effects on the passivity breakdown of copper in chloride‐containing borate buffer solution

2023· article· en· W4388680724 on OpenAlex
Yuting Zhou, Feixiong Mao, Jingkun Yu, Edouard Assellin

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueMaterials and Corrosion · 2023
Typearticle
Languageen
FieldMaterials Science
TopicCorrosion Behavior and Inhibition
Canadian institutionsUniversity of British Columbia
FundersUniversity of British ColumbiaChina Scholarship Council
KeywordsPassivityCopperChlorideOxideCopper oxideChemistryInorganic chemistryCorrosionElectrochemistryBuffer solutionBoronMaterials scienceAnalytical Chemistry (journal)MetallurgyElectrodePhysical chemistryChromatography

Abstract

fetched live from OpenAlex

Abstract Passivity and passivity breakdown of pure copper were studied in alkaline chloride‐containing borate buffer solution from 25°C to 80°C by electrochemical measurements and scanning electron microscopy. The corresponding E –pH diagrams were also calculated. Increased temperatures make the open circuit potential and formation potential for cuprous oxide (Cu 2 O) shift in a negative direction. The mean breakdown potential shifts in a positive direction and the distribution of breakdown potential has a wider width, while the minimum breakdown potential decreases slightly at higher temperature. The anodic passive film formed at 0.4 V versus Ag/AgCl for 6 h in a chloride‐free solution at T ≥ 40°C can maintain passivity after the addition of 0.1 M NaCl, but cannot maintain passivity at 25°C at the same concentration. High temperature benefits the growth of copper oxide over the formation of copper chloride species. Cu 2 O and CuO have excellent corrosion resistance to 0.1 M NaCl and passivity can be maintained well above the CuO/Cu 2 O equilibrium at pH > 8.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.023
Threshold uncertainty score0.394

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.239
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it