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Record W4388974474 · doi:10.1680/jenes.23.00090

Thiol-modified olive-stone biochar preparation for Hg(II) removal from aqueous solutions

2023· article· en· W4388974474 on OpenAlexvenueno aff
Mery-Cecilia Gomez-Marroquin, Dalia Carbonel, Stephanie Esquivel, Henry A. Colorado

Bibliographic record

VenueJournal of Environmental Engineering and Science · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsnot available
Fundersnot available
KeywordsBiocharAdsorptionPyrolysisMercury (programming language)Aqueous solutionChemistryThiolCharcoalEnvironmental remediationEnvironmental chemistryNuclear chemistryContaminationOrganic chemistry

Abstract

fetched live from OpenAlex

Mercury (Hg) is a heavy metal whose toxicity poses significant environmental and health risks. Utilising biochar prepared from biomass waste is a straightforward and effective method for removing mercury from water. This research centred on producing a thiol-functionalised biochar derived from olive-stone waste for the removal of mercury (II) from aqueous solutions. Characterisation analyses confirmed successful functionalisation. The biochar, despite having a limited specific surface area (4.14 m 2 /g) due to raw material nature and pyrolysis conditions, exhibited a notable ability for mercury (II) adsorption, primarily attributed to the thiol-modified surface. Adsorption was assessed using a 2 3 factorial design, with the variables being adsorption time, biochar dose and initial mercury (II) concentration in the solution. Biochar dose emerged as the most influential factor, followed by adsorption time and, lastly, initial mercury (II) concentration. The peak removal efficiency of the model stood at 98.19%. The kinetics aligned with the pseudo-first-order and intraparticle diffusion models, suggesting a surface adsorption mechanism coupled with pore diffusion. This work accentuates the potential of olive-derived biochar, when thiol enhanced, in treating aqueous systems contaminated with mercury (II).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.888
Threshold uncertainty score0.426

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.229
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2023
Admission routes1
Has abstractyes

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