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Cobalamin‐deficiency results in altered partitioning of mitochondrial one‐carbon units to formate

2017· article· en· W4389020680 on OpenAlexafffundabout
Luke MacMillan, Garrett Tingley, Margaret E. Brosnan, John T. Brosnan

Bibliographic record

VenueThe FASEB Journal · 2017
Typearticle
Languageen
FieldMedicine
TopicFolate and B Vitamins Research
Canadian institutionsMemorial University of Newfoundland
FundersCanadian Institutes of Health ResearchMemorial University of NewfoundlandResearch and Development Corporation of Newfoundland and Labrador
KeywordsFormateSerineChemistryBiochemistryMethionineMitochondrionMetabolismSarcosineBiologyAmino acidGlycineEnzyme

Abstract

fetched live from OpenAlex

Vitamin B 12 , a co‐factor for methionine synthase, plays an important role in folate‐dependent remethylation of homocysteine. We have shown that cobalamin deficiency results in a marked elevation in plasma formate. De novo production of formate in rats was determined as described by Morrow et al (JBC 2015). Formate production from one‐carbon precursors by isolated rat liver mitochondria was measured by GC‐MS. 14 CO 2 production from 3‐[ 14 C]‐serine by isolated rat liver mitochondria, expression of key genes (RT‐qPCR) and changes in protein expression (immunoblot) were also determined. Vitamin B 12 ‐deficient rats (B 12 ‐def) showed a 55% increase in endogenous formate production, consistent with the elevated formate levels. Formate production by isolated mitochondria from serine, dimethylglycine, and sarcosine was increased by at least 60% in B 12 ‐def animals while 14 CO 2 production from serine by these mitochondria was 26% lower compared to replete controls. The expression of Mthfd1l in B 12 ‐def animals was unchanged but the expression of Aldh1l1 and Aldh1l2 was reduced by 40–60% of that in the livers of control animals. We suggest that the partitioning of mitochondrial formyl‐THF between oxidation to CO 2 (by ALDH1L2) and production of free formate (by MTHFD1L) is a key control point in one‐carbon metabolism. In B 12 ‐def the decreased flux through ALDH1L2, in the face of a constant rate of 10‐formyl‐THF disposition can explain the increased production and increased concentration of formate. We speculate that the decreased hepatic SAM levels found in B 12 ‐def animals may cause increased production of one‐carbon groups in the form of formate to replenish hepatic SAM. Since mitochondrial formate becomes available to the cytosol we suggest that this metabolic bifurcation may regulate the entry of formate into the cytosolic one‐carbon pool. Support or Funding Information Supported by CIHR, RDC, and Memorial University of Newfoundland

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.073
GPT teacher head0.334
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2017
Admission routes3
Has abstractyes

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