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Record W4389058427 · doi:10.1021/acsnano.3c10218

Above-Room-Temperature Strong Ferromagnetism in 2D MnB Nanosheet

2023· article· en· W4389058427 on OpenAlexaff
Yong Wang, Wei Xu, Dingyi Yang, Yu Zhang, Yongjie Xu, Zixuan Cheng, Xuke Mi, Yizhang Wu, Yan Liu, Yue Hao, Genquan Han

Bibliographic record

VenueACS Nano · 2023
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsInstitut National de la Recherche Scientifique
FundersNational Key Research and Development Program of ChinaNatural Science Basic Research Program of Shaanxi ProvinceNatural Science Foundation of Zhejiang ProvinceFundamental Research Funds for the Central UniversitiesNational Postdoctoral Program for Innovative TalentsNational Natural Science Foundation of China
KeywordsNanosheetSpintronicsFerromagnetismMaterials scienceCondensed matter physicsCurie temperatureMagnetic momentDensity functional theoryMagnetocrystalline anisotropyMagnetic anisotropyNanotechnologyMagnetizationMagnetic fieldPhysicsChemistryComputational chemistry

Abstract

fetched live from OpenAlex

Two-dimensional (2D) room-temperature (RT) ferromagnetic materials have amassed considerable interest in the field of fundamental physics for applications in next-generation spintronic devices owing to their physical properties. However, realizing strong RT ferromagnetism and a high Curie temperature ( T C ) in these 2D magnetic materials remains challenging. Herein, we develop a 2D MnB nanosheet for known 2D ferromagnets that demonstrates strong RT ferromagnetism and a record-high above-RT T C of ∼585.9 K. Through magnetic force microscopy, clear evidence of ferromagnetic behavior is observed at room temperature. Structural characterization and density functional theory calculations further reveal that (i) after exfoliation of bulk, −OH functional groups were introduced in addition to Mn–B bonds being formed, which increases MnB nanosheet T C to 585.9 K and (ii) the d 3 ↑ spin configuration of Mn mainly contributed to the magnetic moment of MnB, and the hybridization between the d xz (d yz ) and d z 2 orbitals of the Mn atom provides a large contribution to magnetic anisotropy, which stabilizes the magnetic property of MnB. Our findings establish a strong experimental foundation for 2D MnB nanosheets as ideal materials for the construction of spintronic devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.261
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2023
Admission routes1
Has abstractyes

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