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Record W4389237597 · doi:10.1002/macp.202300282

Evaluation of Doped Polyaniline as Potential Sensing Materials and/or Absorbents For Styrene and Phthalates in Aqueous Solutions

2023· article· en· W4389237597 on OpenAlexaff
D. Reese Tourne, Jordan Jones, Alex J. Atwater, Katherine M. E. Stewart

Bibliographic record

VenueMacromolecular Chemistry and Physics · 2023
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsTrent University
FundersNational Institute of Standards and Technology
KeywordsPolyanilineStyreneSelectivityAqueous solutionPlasticizerMaterials scienceSorptionChemical engineeringTitanium dioxideDibutyl phthalatePolymerConductive polymerOxideChemistryCopolymerOrganic chemistryPolymerizationAdsorptionComposite material

Abstract

fetched live from OpenAlex

Abstract The removal and detection of toxic analytes, including monomers and plasticizers, is important for both health and the environment. Potential absorbents and/or sensing materials are successfully made from polyaniline (PANI) and PANI doped with 10 wt.% of aluminum oxide (PANI‐Al 2 O 3 ) and titanium dioxide (PANI‐TiO 2 ). The amount of metal oxide incorporated into the surface layers of the polymer and the total amount incorporated are confirmed by energy dispersive X‐rays (EDX) and microwave plasma‐ atomic emission spectroscopy (MP‐AES), respectively. All three materials are evaluated as potential sensing materials and/or absorbents for styrene, monobutyl phthalate (MBP), and dibutyl phthalate (DBP) at 100 ppm in aqueous solutions. It is found that incorporating TiO 2 into PANI improved both the sensitivity and selectivity to styrene, making PANI‐TiO 2 a good absorbent and potential sensing material for styrene. Additionally, incorporating Al 2 O 3 into PANI improved the sorption to MBP, but reduced the selectivity. As a proof‐of‐concept, the responses of the polymeric nanocomposites are combined and analyzed using principal component analysis (PCA) as such an algorithm. The output reveals good separation of the responses to each analyte, thereby demonstrating how sensing materials with poorer selectivity can be used together to overcome limitations in selectivity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.331

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.038
GPT teacher head0.308
Teacher spread0.270 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes1
Has abstractyes

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