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Record W4391233587 · doi:10.1088/0026-1394/61/1a/08002

Final report for SIM.QM-S12: supplementary comparison for trace elements in natural water

2024· article· en· W4391233587 on OpenAlexaff
Patrícia Grinberg, Kenny Nadeau, Lu Yang, Zoltán Mester, Wai-hong Fung, Chun-wai Tse, Jeffrey Merrick, Ian White, Isaac Schipp, Osvaldo Reyes Acosta, Mabel Puelles, Jose Luis Gonzales Quino, Rodrigo Caciano de Sena, Marcelo Dominguez de Almeida, Emily Silva Dutra, Jingbo Chao, Dong Lijie, Elias Kakoulides, G Karanikolopoulos, E Stathoudaki, S. Swarupa Tripathy, Dibya Dolridge Toppo, Jyoti Pokhariyal, A. G. Gopala Krishna, Chinky Vinod, Lakhan Taneja, Christine Elishian, Isna Komalasari, Norliza Baharom, Haslina Binti Abdul Kadir, Elmer Carrasco Solis, Christian Uribe, Alleni T Junsay, Christian D. Laurio, Johnester D Maniego, Clarissa J. Gatchalian, Jan-Ervin C Guerrero, Michał Strzelec, Anna Bojanowska-Czajka, Beata Warzywoda, Radojko Jačimović, Tea Zuliani, Pranee Phukphatthanachai, Nunnapus Laitip, Usana Thiengmanee, Romina Napoli, Elizabeth Ferreira

Bibliographic record

VenueMetrologia · 2024
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsTRACE (psycholinguistics)QM/MMComputer sciencePhysicsPhilosophyMolecular dynamicsQuantum mechanics

Abstract

fetched live from OpenAlex

Main text The SIM Supplementary Comparison SIM.QM-S12 for Trace Elements in Natural Water was undertaken to assess and demonstrate the analytical capabilities of national metrology institutes (NMIs) and designated institutes (DIs) of SIM members (or other regions) for the accurate determination of trace elements in natural water at µg/kg levels. Evidence of successful participation in formal, relevant international comparisons is needed to document calibration and measurement capability claims (CMCs) made by NMIs and DIs. Seventeen NMIs and DIs participated. Participants were requested to evaluate the mass fractions, expressed in µg/kg, of arsenic, cadmium, lead and antimony in a natural mineral groundwater that was spiked with the respective elements. A variety of instrumental techniques including inductively coupled plasma mass spectrometry (ICP-MS), isotope dilution ICP-MS (ID-ICP-MS), inductively coupled plasma optical emission spectrometry (ICP-OES), electrothermal atomic absorption spectrometry (ETAAS) and hydride generation flame atomic absorption spectrometry (HG-FAAS) were used by the participants for the determination. The NIST decision tree was used to assign the SCRV estimate for the proposed measurands and to calculate the degrees of equivalence of each national measurement standard following the IAWG Guidance on Using NIST Decision Tree for Comparison Reporting from 30 June 2023. Successful participation in SIM.QM-S12 demonstrates measurement for determination of elements in water matrices. Considering the IAWG Core Capability Matrix, this material falls into the matrix challenge called "Water/aqueous", which corresponds to the CCQM amount-of-substance category fresh water, and so will support CMCs for the metalloids and semi-metals at mass fraction levels below 50 µg/kg (As and Sb measurements) and transition elements at mass fraction levels below 50 µg/kg (except Hg) (for Cd and Pb measurements). To reach the main text of this paper, click on Final Report . Note that this text is that which appears in Appendix B of the BIPM key comparison database https://www.bipm.org/kcdb/ . The final report has been peer-reviewed and approved for publication by the CCQM, according to the provisions of the CIPM Mutual Recognition Arrangement (CIPM MRA).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.242
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.056
GPT teacher head0.369
Teacher spread0.313 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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