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Record W4391299744

Flare Carbon Conversion Efficiency Quantification using a Long Wave Infrared Fourier Transform Spectrometer

2024· preprint· en· W4391299744 on OpenAlexafffund
Paule Lapeyre, Sriram Narayanan, Martin Larivière-Bastien, Kyle J. Daun

Bibliographic record

VenueHAL (Le Centre pour la Communication Scientifique Directe) · 2024
Typepreprint
Languageen
FieldEnergy
TopicOil, Gas, and Environmental Issues
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsFourier transformFlareFourier transform infrared spectroscopyInfraredSpectrometerFourier transform spectroscopyCarbon fibersMaterials sciencePhysicsOpticsAstrophysicsComposite number
DOInot available

Abstract

fetched live from OpenAlex

In recent years, measuring emissions from flares has assumed new significance due to the high global warming potential of these species and the enormous volumes of gases flared, coupled with doubt regarding the 98% combustion efficiency (CE) estimate often used to assess the impact of flaring on climate change. Hyperspectral cameras are a particularly promising avenue since they can directly visualize the species column density contained within the entire flare plume via the absorption features of these species over the infrared spectrum. Imaging Fourier transform spectrometers (IFTS) generate a datacube of images, each of these pertain to a unique wavelength. Spectroscopic and velocity submodels are then used to obtain the species mass flow rates needed to calculate the CE. This work compares the performance of mid-wavelength infrared (MWIR) and long-wavelength infrared (LWIR) IFTSs for measuring the CE for flares at petrochemical refineries, and, for the first time, uses a LWIR IFTS to fingerprint the plume species and estimate the CE. While the MWIR camera covers prominent CO2 features, the limited dynamic range of the camera can induce lens flare artifacts originating in the combustion zone that bias quantification of the CO2 in the downstream plume. Images from the LWIR camera, in contrast, are free of these artifacts, and the dynamic range is sufficient to measure unburned fuel, key to accurate CE estimates.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.438
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.225
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes2
Has abstractyes

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