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Record W4391614170 · doi:10.1002/adom.202302651

Polarization‐Sensitive and Self‐Driven Pyro‐Phototronic Photodetectors Based on MoS<sub>2</sub>‐Water Heterojunctions

2024· article· en· W4391614170 on OpenAlex
Amin Abnavi, Ribwar Ahmadi, Hamidreza Ghanbari, Mirette Fawzy, Mohammad Reza Mohammadzadeh, Fahmid Kabir, Michael M. Adachi

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Optical Materials · 2024
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsSimon Fraser University
FundersWestern Economic Diversification CanadaBritish Columbia Knowledge Development FundCMC MicrosystemsNatural Sciences and Engineering Research Council of CanadaSimon Fraser UniversityCanada Foundation for Innovation
KeywordsPhotodetectorMaterials scienceOptoelectronicsResponsivityHeterojunctionSpecific detectivityPolarization (electrochemistry)Electric fieldOpticsPhysics

Abstract

fetched live from OpenAlex

Abstract Polarization‐sensitive and self‐driven pyroelectric‐based photodetectors have recently gained interest due to their potential application in artificial electronic eyes, biomedical imaging, and optical switches. Here, a photodetector based on light modulation‐induced polarization and depolarization of water molecules on the surface of a 2D MoS 2 crystal is reported. The MoS 2 ‐water heterostructure photodetector serves as a self‐driven pyro‐phototronic device that converts light‐induced thermal energy to electrical signals, leading to a transient photoresponsivity as high as 24.6 mA W −1 and a specific detectivity of 2.85 × 10 8 Jones under 470 nm wavelength at zero bias. Due to the formation of a built‐in electric field at the MoS 2 ‐water interface, this structure also has a high steady–state responsivity of 3.62 A W −1 and detectivity of 9.18 × 10 8 Jones at 3 V bias, along with a fast response time of ≈0.74 ms. Moreover, due to the rearrangement of the hydrogen bond network in the liquid water upon visible light illumination, the MoS 2 ‐water photodetector is light polarization‐sensitive. The simple fabrication process, low cost, polarization sensitivity, and high performance of the MoS 2 ‐water structure make it an excellent candidate for liquid‐compatible photodetectors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.227
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it