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Record W4392551488 · doi:10.26434/chemrxiv-2024-z8blq

The role of fine particles in the stability of emulsion in the naphthenic froth treatment (NFT) process

2024· preprint· en· W4392551488 on OpenAlexaff
Arian Velayati, Hongbo Zeng

Bibliographic record

VenueChemRxiv · 2024
Typepreprint
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of AlbertaNorthern Alberta Institute of Technology
Fundersnot available
KeywordsEmulsionNaphthenic acidProcess (computing)Stability (learning theory)Materials scienceEnvironmental scienceEngineeringChemical engineeringMetallurgyComputer science

Abstract

fetched live from OpenAlex

This study investigates the role of fine particles in stabilizing emulsion in the naphthenic froth treatment (NFT) process. The characterization results of different types of solids collected from the diluted bitumen froth indicate that kaolinite is the dominant clay mineral in the composition of NFT solids. There were differences in the mineralogy of the fine samples depending on the phase (carrier fluid) from which the samples were collected. FTIR analysis shows that the fines that remain in the diluted bitumen even after several hours of sample retention time are mainly kaolinite, though the presence of other minerals such as siderite is very likely. Moreover, the presence of organic functional groups on the surface of the particles is confirmed for all types of solids in the FTIR analysis, regardless of the washing and drying procedures employed. Inspection of the different layers of the diluted bitumen via micrography and measurement of the solids concentration shows higher fine content and smaller particles in the top layer, a dire situation for destabilizing the emulsion in the top layer, supported by the observation that the water droplets in this layer are tiny. Solid partitioning tests revealed the solid particles migrate to the interfacial region and the aqueous phase. The concentration of particles increased in the interfacial region with the presence of asphaltene in the oil phase (dominant effect) and the increased polarity of the oil. The wettability measurements show that without the coverage of solid particles with organics (asphaltene-resin molecules), the fine particles are extremely hydrophilic. The adsorption of asphaltene-resin matter on the fine particles increased the hydrophobicity of the fines, a situation that promotes the partitioning of the fine particles at the interfacial region and the stability of the droplets. It was observed that the contact angle increased with the decreasing polarity of the oil phase. In the interfacial tension measurements, the fine solids with minimal asphaltic matter coverage did not remain suspended in the oil phase and either sedimented rapidly or migrated to the air-oil interface, unlike the organics-covered solids which remained immersed in oil. No decrease in the interfacial tension was recorded for the water-oil systems in the presence of fine solids. Interfacial rheology measurements illustrate the viscoelastic behavior of the interfacial film at lower frequencies and higher fine particle concentrations. We conclude that if not for the interaction between the asphaltic matter and the fine particles, the emulsion stability by fine particles would have been very unlikely.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.275
Teacher spread0.257 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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