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Record W4392584281 · doi:10.5194/egusphere-egu24-6160

Why nanoplastics do not enhance the transport of contaminants in the critical zone

2024· preprint· en· W4392584281 on OpenAlexaff
Thilo Hofmann, Charlotte Henkel, Thorsten Hueffer, Stephanie Castan

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEnvironmental Science
TopicMicroplastics and Plastic Pollution
Canadian institutionsMcGill University
Fundersnot available
KeywordsContaminationEnvironmental scienceBiochemical engineeringChemistryBiologyEngineeringEcology

Abstract

fetched live from OpenAlex

The impact of nanoplastics on the co-transport of emerging contaminants is a subject of ongoing debate. Agricultural soils face potential contamination from micro- and nanoplastics through diverse agricultural practices. Various authors argue that the substantial surface area of small particles and their high sorption potential may considerably augment the mobility of numerous contaminants within the critical zone. Concerns have been expressed regarding the role of micro- and nanoplastics as carriers for organic contaminants into deeper soil layers, posing a potential threat to groundwater resources, particularly in agricultural soils where sewage sludge and plant protection products are frequently applied.In this study, we investigated the correlation between transport and desorption timescales by employing two diffusion models for micro- and nanoplastics ranging from 100 nm to 1 mm. To assess the transport of contaminants bound to these plastics, we examined the diffusion and partitioning coefficients of prominent agrochemicals and additives, along with commonly used polymers like polyethylene and tire material. Our modeling analysis reveals that the desorption rate of most organic contaminants is too rapid for micro- and nanoplastics to serve as effective transport facilitators in soil. Notably, the transport of contaminants facilitated by microplastics was observed to be significant only for highly hydrophobic contaminants under preferential fast-flow conditions.While micro- and nanoplastics could potentially introduce harmful contaminants into agricultural soils, our study suggests they do not significantly enhance contaminant mobility. Importantly, we found that nanoplastics, in particular, do not promote contaminant relocation under conditions relevant to almost all contaminants of concern.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.002
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.248
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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