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Record W4392585484 · doi:10.5194/egusphere-egu24-4590

Triple sulfur isotope constraints on the sulfur cycling in Lake Sevan, Armenia

2024· preprint· en· W4392585484 on OpenAlexaff
Alexey Kamyshny, Khoren Avetisyan, Natella Mirzoyan, R. Kelly Payne

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEarth and Planetary Sciences
TopicMarine and environmental studies
Canadian institutionsThe Scarborough HospitalUniversity of Toronto
Fundersnot available
KeywordsSulfurCyclingIsotopeEnvironmental chemistryEnvironmental scienceChemistryGeographyPhysicsArchaeologyOrganic chemistryNuclear physics

Abstract

fetched live from OpenAlex

Lake Sevan is a meso-eutrophic water body, which was severely impacted by anthropogenic level decrease, pollution and eutrophication during the last century. Starting in the 1970s, a decrease in the water level and an increase in dissolved inorganic nitrogen concentrations resulted in oxygen depletion in the hypolimnion of the lake during summer–autumn thermal stratification of the water column. Our work shows that in October 2019, the redox conditions in the hypolimnion progressed not only to full depletion of oxygen and nitrate, but to the formation of a hydrogen sulfide-rich deep-water layer, which covers 66% of lake’s bottom and accounts for 19% of its water volume. Concentrations of hydrogen sulfide in the hypolimnion of Major and Minor Sevan in October were as high as 9 and 39 μM, respectively.Triple sulfur isotope composition of sulfate and hydrogen sulfide in the water column of the lake provides further constraints on the biogeochemical processes which result in the formation of hydrogen-sulfide hypolimnion. Values of δ34S for hypolimnetic sulfide are lower by only 7–12 ‰ compared to epilimnetic sulfate, while δ33S values of sulfide are similar to the δ33S values of sulfate. These isotopic fingerprints are not consistent either with microbial sulfate reduction in the water column or with its combination with re-oxidative sulfur cycle as the sources of hydrogen sulfide in the hypolimnion. We attribute the formation of a sulfidic deep-water layer to a combination of microbial sulfate reduction in the water column and diffusion of hydrogen sulfide from the sediments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.056
Threshold uncertainty score0.111

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0010.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.221
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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