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Record W4393032697 · doi:10.1103/physrevb.109.094113

Thermal equation of state of rhodium to 191 GPa and 2700 K using double-sided flash laser heating in a diamond anvil cell

2024· article· fi· W4393032697 on OpenAlexfundno aff
J. McHardy, C. V. Storm, M. J. Duff, Cameron Lonsdale, Gavin Woolman, M. I. McMahon, Nico Giordano, Simon G. MacLeod

Bibliographic record

VenuePhysical review. B./Physical review. B · 2024
Typearticle
Languagefi
FieldEarth and Planetary Sciences
TopicHigh-pressure geophysics and materials
Canadian institutionsnot available
FundersDeutsches Elektronen-SynchrotronEngineering and Physical Sciences Research CouncilEuropean Synchrotron Radiation FacilityEnvironmental Studies Research FundsHelmholtz-Gemeinschaft
KeywordsFlash (photography)LaserRhodiumMaterials scienceDiamond anvil cellEquation of stateDiamondThermalAtomic physicsOpticsPhysicsThermodynamicsDiffractionChemistryComposite material

Abstract

fetched live from OpenAlex

The phase behavior of rhodium (Rh) metal has been studied to 191 GPa and 2700 K using a combination of room-temperature isothermal compression and double-sided flash laser heating experiments. The isothermal compression data have been fitted with a second-order adapted polynomial of order L equation of state (EoS) with best-fitting parameters of V0=13.764(2)Å3/atom , K0=258(3)GPa, and K′=5.36(9) . Two-dimensional maps of the uniaxial stress component t are presented for Rh at different pressures showing the spatial distribution of the local stress state of a relatively high-yield strength material encased in a Bi pressure medium. In addition, a simple, thermal pressure equation-of-state model, based on a single Einstein temperature, has been fitted to the high-pressure-temperature data up to 2700 K at 148 GPa and ambient-pressure thermal expansion data up to 1982 K. Also determined are the best-fitting parameters to reproduce the thermal EoS within the two-dimensional integration software. The optimized parameters are V0=13.764Å3/atom , K0=260.54GPa , K′=5.114 , αT=2.99×10−5 K−1 , ∂αT/∂T=1.27×10−9 K−2 , ∂K0/∂T=−6.43×10−5GPa/K , and ∂K′/∂T=−9.3×10−10K−1 . Published by the American Physical Society 2024

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.032
GPT teacher head0.331
Teacher spread0.299 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2024
Admission routes1
Has abstractyes

Explore more

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