MétaCan
Menu
Back to cohort
Record W4393153334 · doi:10.21203/rs.3.rs-3894488/v1

Evaluation of a customized reactive nanoscale-zero-valent iron and zeolite thin capping blend for enhancing natural recovery of wetlands impacted by contaminated legacy gold mine tailings

2024· preprint· en· W4393153334 on OpenAlexfundaboutno aff
E. Emily V. Chapman, Linda M. Campbell

Bibliographic record

VenueResearch Square · 2024
Typepreprint
Languageen
FieldEngineering
TopicEnvironmental remediation with nanomaterials
Canadian institutionsnot available
FundersEnvironment and Climate Change CanadaHellenic Ministry of Rural Development and Food
KeywordsTailingsZerovalent ironZeoliteNatural (archaeology)WetlandNanoscopic scaleMining engineeringEnvironmental scienceContaminationMaterials scienceWaste managementEnvironmental engineeringGeologyMetallurgyNanotechnologyEngineeringChemistryEcologyCatalysis

Abstract

fetched live from OpenAlex

Abstract Legacy gold mine tailings from the 1800’s in Nova Scotia, Canada have elevated mercury (Hg) and arsenic (As) concentrations. Tailings, were slurried into wetlands without treatment. Over a century later, those impacted wetlands are still at risk and innovative in-situ treatment approaches to support natural biological and chemical recovery are needed. Here we report results of our proof-of-concept laboratory study with a customized reactive thin layer capping to limit mobility, bioaccumulation and toxicity of Hg and As in wetland sediment impacted by legacy tailings. The customized reactive amendment is a blend of NANOFER STAR nanoscale zero valent iron (nZVI) and fine-grained zeolite (clinoptilolite) inserted either below, or within a thin cap (silica sand, bentonite and zeolite) and placed over contaminated wetland sediments in beakers. Due to the high concentrations of Hg and As in sediments, invertebrates ( Hyalella azteca , Daphnia magna and Caridina multidente) exposed to untreated wetland sediment exhibited high mortality and bioaccumulation of Hg. The reactive capping applications improved the survival of H. azteca and D. magna similar to the survival rates seen in our clean control sediment. Bioaccumulation of Hg was also reduced in C. multidente exposed to the treated sediment compared to the untreated sediment. Furthermore, total [Hg] and [As] in the overlaying water of treated contaminated sediments were reduced by 88% and 99% respectively. Our proof-of-concept testing of this reactive capping blend shows potential for managing and supporting natural recovery of wetlands impacted by historical gold-mine tailings.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.005
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.074
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0050.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.323
Teacher spread0.299 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes2
Has abstractyes

Explore more

Same venueResearch SquareSame topicEnvironmental remediation with nanomaterialsFrench-language works237,207