MétaCan
Menu
Back to cohort
Record W4393277585 · doi:10.1002/smtd.202301695

Harnessing the Synergetic Effects of Ag, Mn Dopants in Eco‐Friendly Ultraviolet Selective Quantum Dots for Luminescent Solar Concentrators

2024· article· en· W4393277585 on OpenAlexafffund
Lei Jin, Ehsan Hamzehpoor, Gurpreet Singh Selopal, Jiabin Liu, Pawan Kumar, Daniele Benetti, Xin Tong, Zhiming M. Wang, Federico Rosei

Bibliographic record

VenueSmall Methods · 2024
Typearticle
Languageen
FieldMaterials Science
TopicQuantum Dots Synthesis And Properties
Canadian institutionsDalhousie UniversityMcGill UniversityInstitut National de la Recherche Scientifique
FundersNational Key Research and Development Program of ChinaFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of CanadaSichuan Province Science and Technology Support ProgramChina Postdoctoral Science FoundationCanada Foundation for InnovationNational Natural Science Foundation of ChinaCanada Research ChairsNational Science Foundation
KeywordsQuantum dotPhotoluminescenceMaterials scienceUltravioletColor rendering indexVisible spectrumDopantLuminescenceQuantum yieldOptoelectronicsNanotechnologyOpticsLight-emitting diodeDopingFluorescencePhysics

Abstract

fetched live from OpenAlex

Abstract Quantum dots (QDs) are promising building blocks for luminescent solar concentrators (LSCs), yet most QD‐based LSCs suffer from toxic metal composition and color tinting. UV‐selective harvesting QDs can enable visible transparency, but their development is restricted by large reabsorption losses and low photoluminescence quantum yield (PLQY). The developed here Ag, Mn: ZnInS2/ZnS QDs show a high PLQY of 53% due to the passivating effect of ZnS shell. These QDs selectively absorb UV light and emit orange‐red light with a large Stokes shift of 180 nm. A LSC of 5 × 5 × 0.2 cm3, fabricated using a poly(lauryl methacrylate) (PLMA) as a matrix, maintains 87% of integrated PL after 7 h of UV exposure. The QD‐PLMA achieved 90.7% average visible transparency (AVT) and a color rendering index (CRI) of 95.8, which is close to plain PLMA (AVT = 90.8%; CRI = 99.5), yielding excellent visible light transparency. Incorporating Si‐PVs at LSC edges, the Ag, Mn: ZIS/ZnS QD‐LSC achieved an optical efficiency of 1.42%, ranking competitively among high‐performing UV‐harvesting LSCs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.319
Teacher spread0.293 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2024
Admission routes2
Has abstractyes

Explore more

Same venueSmall MethodsSame topicQuantum Dots Synthesis And PropertiesFrench-language works237,207