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Record W4394603854 · doi:10.1021/acsanm.4c01143

Porous Nanostructured Chromium-Doped Tungsten Oxide Electrocatalysts for Flutamide and Nilutamide Detection

2024· article· en· W4394603854 on OpenAlexaff
Mahesh M. Shanbhag, Shankara S. Kalanur, Abdullah N. Alodhayb, Nagaraj P. Shetti

Bibliographic record

VenueACS Applied Nano Materials · 2024
Typearticle
Languageen
FieldEngineering
TopicElectrochemical sensors and biosensors
Canadian institutionsUniversité du Québec à Trois-Rivières
FundersScience and Engineering Research BoardMinistry of Education – Kingdom of Saudi Arabi
KeywordsMaterials scienceCyclic voltammetryElectrochemical gas sensorX-ray photoelectron spectroscopyElectrochemistryAnalytical Chemistry (journal)NanotechnologyNuclear chemistryChemical engineeringChemistryElectrodeOrganic chemistryPhysical chemistry

Abstract

fetched live from OpenAlex

In the present study, an electrochemical sensor based on a Cr-doped WO 3 nanostructure was designed and exploited for pharmaceutical drug analysis. Cr-doped WO 3 nanostructures were prepared by treating the W and Cr precursors with hydrothermal condensation. A thorough characterization was conducted for structural and elemental insights using scanning electron microscopy, X-ray powder diffraction, transmission electron microscopy, and X-ray photoelectron spectroscopy methods. The optimized electrochemical response was obtained with 1.68 atom % of Cr in the WO 3 lattice. The developed nanoparticles were employed in the electrochemical detection of antiandrogen drugs such as flutamide (FLTM) and nilutamide (NLTM) using cyclic voltammetry and square wave voltammetry techniques. The developed sensor was employed to evaluate the physiochemical and thermodynamical parameters of the voltammetric process by investigating the effect of scan rates and temperatures on the quasi-reversible signals of FLTM and NLTM. The Cr-WO 3 /CPE shows a sensitivity of 24.9 and 49.1 μA μM –1 cm –2 for FLTM and NLTM with detection limits of 4.2 and 3.07 nM, respectively. The sensor was employed to detect the desired drug moiety in the urine samples (real and synthetic) and pharmaceutical drugs; the good recovery values demonstrating the applicability and selectivity of the sensor were supported by excipient interference investigation. Thus, the developed sensor and methods hold potential for future research in identifying additional bioactive molecules in pharmaceutical and clinical trials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.187
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2024
Admission routes1
Has abstractyes

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