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Record W4394717799 · doi:10.1002/adfm.202403448

Fenton Reaction Doubled Biomass Carbon Activation Efficiency for High‐Performance Supercapacitors

2024· article· en· W4394717799 on OpenAlexaff
Yanyu Li, Lifeng Ni, Jiayan Luo, Lulu Zhu, Xiaoxiao Zhang, Hongjie Li, Imran Zada, Jin Yu, Shenmin Zhu, Keryn Lian, Yao Li, Di Zhang

Bibliographic record

VenueAdvanced Functional Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsUniversity of Toronto
FundersKey Technologies Research and Development Program
KeywordsSupercapacitorMaterials scienceElectrolyteCapacitanceCarbon fibersChemical engineeringBiomass (ecology)ElectrochemistryStack (abstract data type)Power densitySpecific energyElectrodeNanotechnologyComposite materialChemistryPhysical chemistryThermodynamics

Abstract

fetched live from OpenAlex

Abstract The huge consumption of alkali during biomass‐derived porous carbon production leads to pollution and high carbon‐emission. This study employs the concept of Fenton chemistry to achieve hierarchical porous biomass carbon materials with a remarkably high specific surface area of 3440 m 2 g −1 with double activation efficiency compared to traditional activation process. The optimized carbon electrode demonstrates exceptional specific capacitance of 425.2 F g −1 at a current density of 0.1 A g −1 and great rate performance (286.1 F g −1 at 100 A g −1 ) in 6 m KOH electrolyte. The enabled supercapacitor demonstrates remarkable cycling stability, retaining up to 99.74% of its initial capacitance after undergoing 20 000 charge–discharge cycles. In addition, the electrolyte ion distribution in different pore structures is simulated using Molecular Dynamics, which confirms that the structure is conducive to the rapid diffusion of ions, thus matching the excellent electrochemical properties. The assembled symmetric supercapacitors achieve a maximum energy density of 42.1 Wh kg −1 (12.1 Wh kg −1 based on cell stack mass) in TEABF 4 /AN electrolyte. This work presents an effective technique for the formation of porous structures from biomass precursors. The novel methodology can be applied to many other similar systems for energy storage and beyond.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.239
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations146
Published2024
Admission routes1
Has abstractyes

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