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Record W4394857920 · doi:10.1016/j.chemgeo.2024.122093

Phosphorus dynamics in an ice-covered lake: Insights from geochemical gradients in water and sediments

2024· article· en· W4394857920 on OpenAlexafffund
Md. Samrat Alam, Arthur Zastepa, Maria Dittrich

Bibliographic record

VenueChemical Geology · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicAquatic Ecosystems and Phytoplankton Dynamics
Canadian institutionsThe Scarborough HospitalEnvironment and Climate Change CanadaUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsWater columnBiogeochemical cycleGeologySedimentPore water pressureSediment–water interfaceCyclingSurface waterHydrology (agriculture)Stratification (seeds)Hypoxia (environmental)Bottom waterEnvironmental chemistryOceanographyGeomorphologyEnvironmental scienceOxygenChemistry

Abstract

fetched live from OpenAlex

Understanding the role of seasonally ice-covered lakes in biogeochemical cycling is important for predicting the effects of changing winter conditions. However, little is known about phosphorus (P) cycling and the mechanisms of internal P release in seasonally ice-covered lakes. We investigated under-ice P cycling in a large and temperate lake composed of several basins with significantly different water depths. We used a multifaceted approach, combining analyses of P and total iron (Fe) distributions in sediments, pore water, and the water column. During the winter period, steep gradients of redox-sensitive parameters (i.e., O2 and Eh) formed at the sediment-water interface (SWI) due to minimal water movement and water column hypoxia. P diffusive fluxes during winter are substantial (0.2–4.8 mg P/m2/day). Short-term P release in shallow basins is strongly influenced by Fe reduction. In contrast, decoupling of Fe from P in deep basins suggests that hypoxia does not play a major role in short-term P mobilization. The differences in short-term P release mechanisms can be interpreted in terms of basin depth, stability of thermal stratification and time of water mixing. This ultimately influences the behavior of Fe and P, as well as their speciation and concentration in the sediment and water column. The deep basins in LOW contained higher total phosphorus (TP) and total iron (Fe) in sediments and soluble reactive phosphorus (SRP) in deep water compared to shallow basins. In surface sediments, P bound to the redox-sensitive P binding form (BD-P) is the diagenetically reactive P phase, emphasizing strong coupling with ferric Fe. In contrast, calcium carbonate-bound P in surface sediments indicates diagenetic sequestration of P with sediment burial. Overall, this study provides evidence that P cycling remains active in winter, and an understanding of its contribution to the overall ecosystem process is needed to predict how lake ecosystems will behave under climate change.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.804
Threshold uncertainty score0.559

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.206
Teacher spread0.201 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2024
Admission routes2
Has abstractyes

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