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Record W4395114137 · doi:10.1016/j.jechem.2024.04.018

Sustainable ammonia synthesis: An in-depth review of non-thermal plasma technologies

2024· article· en· W4395114137 on OpenAlexafffund
Vahid Shahed Gharahshiran, Ying Zheng

Bibliographic record

VenueJournal of Energy Chemistry · 2024
Typearticle
Languageen
FieldChemical Engineering
TopicAmmonia Synthesis and Nitrogen Reduction
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsPlasmaAmmoniaThermalNonthermal plasmaAmmonia productionMaterials scienceEnvironmental scienceChemistryPhysicsThermodynamicsBiochemistry

Abstract

fetched live from OpenAlex

Ammonia serves both as a widely used fertilizer and environmentally friendly energy source due to its high energy density, rich hydrogen content, and emissions-free combustion. Additionally, it offers convenient transportation and storage as a hydrogen carrier. The dominant method used for large-scale ammonia production is the Haber-Bosch process, which requires high temperatures and pressures and is energy-intensive. However, non-thermal plasma offers an eco-friendly alternative for ammonia synthesis, gaining significant attention. It enables ammonia production at lower temperatures and pressures using plasma technology. This review provides insights into the catalyst and reactor developments, which are pivotal for promoting ammonia efficiency and addressing existing challenges. At first, the reaction kinetics and mechanisms are introduced to gain a comprehensive understanding of the reaction pathways involved in plasma-assisted ammonia synthesis. Thereafter, the enhancement of ammonia synthesis efficiency is discussed by developing and optimizing plasma reactors and effective catalysts. The effect of other feeding sources, such as water and methane, instead of hydrogen is also presented. Finally, the challenges and possible solutions are outlined to facilitate energy-saving and enhance ammonia efficiency in the future.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.003
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.002
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0030.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.227
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations61
Published2024
Admission routes2
Has abstractyes

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