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Dual Promotional Effect of <scp>l</scp>-Tryptophan and 1,3-Dioxane on CO<sub>2</sub> Hydrate Kinetics in Seawater under Static/Unstatic Conditions for Carbon Capture and Storage Application

2024· article· en· W4399598839 on OpenAlexaff
Vikas Dhamu, M. Fahed Qureshi, Nithila Selvaraj, Lauren Ji Yuanmin, Iva Tianhui Guo, Praveen Linga

Bibliographic record

VenueEnergy & Fuels · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicMethane Hydrates and Related Phenomena
Canadian institutionsUniversity of Toronto
FundersCollege of Design and Engineering, National University of SingaporeAgency for Science, Technology and Research
KeywordsSeawaterHydrateChemistryKineticsClathrate hydrateDissociation (chemistry)Artificial seawaterCarbon dioxideNuclear chemistryEnvironmental chemistryInorganic chemistryOrganic chemistryGeology

Abstract

fetched live from OpenAlex

CO 2 hydrates hold promising applications, including as a medium for carbon storage in oceanic sediments, as a result of their high storage capacity. However, the presence of high salinity in sediments is likely to affect the CO 2 hydrate kinetics. To counter this challenge, the CO 2 hydrate formation, dissociation, and deep morphology have been investigated in seawater (SW) under static and non-static conditions. Moreover, the effect of a kinetic promoter [1000 ppm of l -tryptophan ( l -tryp)] and a thermodynamic promoter (5 wt % 1,3-dioxane) and dual promotional effects of kinetic and thermodynamic promoters (1000 ppm of l -tryp + 5 wt % 1,3-dioxane) have also been studied. In situ Raman spectroscopy was used to probe the real-time CO 2 dissolution in seawater in the presence of 1,3-dioxane. The CO 2 uptake in seawater for the static system was estimated to be in the following order (20 h): CO 2 (30.5 ± 5.0 mmol/mol) > CO 2 + 1000 ppm of l -tryp (30 ± 1.20 mmol/mol) > CO 2 + 1,3-dioxane + 1000 ppm of l -tryp (26.2 ± 7.1 mmol/mol) > CO 2 + 1,3-dioxane (21.1 ± 6.1 mmol/mol). In comparison, for the non-static system, the CO 2 uptake in seawater was estimated to be in the following order (20 h): CO 2 + 1000 ppm of l -tryp (67.8 ± 2.20 mmol/mol) > CO 2 + 5 wt % 1,3-dioxane (49.3 ± 7.0 mmol/mol) > CO 2 + 5 wt % 1,3-dioxane + 1000 ppm of l -tryp (42.9 ± 4.8 mmol/mol) > CO 2 (39.5 ± 4.1 mmol/mol).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.029
Threshold uncertainty score0.568

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.221
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations59
Published2024
Admission routes1
Has abstractyes

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