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Record W4400919994 · doi:10.1021/acs.chemmater.4c00966

Three-Dimensional Assembled MXene Architectures in Biomedical Innovations

2024· article· en· W4400919994 on OpenAlexaff
Yuting Cai, Yaxuan Li, Yuxuan Du, Natan Roberto de Barros, Patrick Ryan Galligan, Zhenjing Liu, Yuyin Li, Hoilun Wong, Kenan Zhang, Safoora Khoseavi, Negar Hosseinzadeh Kouchehbaghi, Yangzhi Zhu, Zhengtang Luo

Bibliographic record

VenueChemistry of Materials · 2024
Typearticle
Languageen
FieldMaterials Science
TopicMXene and MAX Phase Materials
Canadian institutionsUniversity of British Columbia
FundersInnovation and Technology CommissionResearch Grants Council, University Grants Committee
KeywordsNanotechnologyMaterials science

Abstract

fetched live from OpenAlex

MXenes, primarily composed of two-dimensional (2D) transition metal carbides/nitrides, have emerged as a research hot spot, particularly in the field of biomedicine, owing to their notable physicochemical properties, functional termini, and intriguing biocompatibilities. However, they suffer from smaller specific surface areas, poor mechanical properties, and a lack of dimensional control. Previous studies have indicated that constructing 2D MXene nanosheets into a three-dimensional (3D) structure can effectively reduce the level of re-aggregation, which can provide a larger specific surface area and stronger physical structural support for various applications. This work provides a systematic and focused review of the latest developments in 3D-assembled MXene for biomedical applications. This review first presents a comprehensive summary of the widely employed strategies for manufacturing 3D-assembled MXene architectures, such as metal ion-induced assembly, metal–organic framework-assisted assembly, carbon materials-assisted assembly, and polymer-assisted assembly. Furthermore, research attention is also directed toward exploring the structure–property relationships of 3D-assembled MXenes for diagnostic applications, i.e., biosensing and bioimaging, and therapeutic applications, i.e., drug delivery and tumor therapy. Finally, opportunities and challenges of the 3D-assembled MXenes have also been outlined. We strongly expect that 3D-assembled MXenes can offer significant benefits in the context of clinical translations for theranostic applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.992

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0090.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.282
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2024
Admission routes1
Has abstractyes

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