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Record W4400986468 · doi:10.1155/2024/9534752

Thermal Ammonia Decomposition for Hydrogen‐Rich Fuel Production and the Role of Waste Heat Recovery

2024· article· en· W4400986468 on OpenAlexaff
Payam Shafie, Alain deChamplain, Julien Lépine

Bibliographic record

VenueInternational Journal of Energy Research · 2024
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen Storage and Materials
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsHydrogen productionWaste managementAmmonia productionAmmoniaProduction (economics)Environmental scienceDecompositionHydrogenThermal decompositionChemistryEngineeringEconomics

Abstract

fetched live from OpenAlex

Hydrogen is an attractive future fuel with the potential to play a crucial role in reducing carbon dioxide emissions, but the major obstacles to implement hydrogen are associated with its storage, transportation, and safety. As a solution, ammonia has been recognized as a promising carbon‐free hydrogen carrier; however, due to the poor combustion performance of ammonia fuel, this review first outlines the significance of on‐site ammonia decomposition to generate CO x ‐free H 2 ‐rich fuel. Furthermore, to demonstrate the potential of this approach in different fields, the main focus of this review is on the pivotal role of integrating waste heat recovery and thermal ammonia decomposition across various industries including power plants, transportation, and industrial furnaces, enabling researchers to gain insights and benefit from the work of each other. As a means to enhance fuel saving and reduce greenhouse gas emissions, two significant methods including thermochemical recuperation and autothermal reforming are investigated considering the impact of several factors like exhaust gas species, temperature, and the performance parameters of the main fuel consumers. Finally, the paper provides vital recommendations for research directions in waste heat recovery‐based ammonia decomposition systems to promote sustainable and eco‐friendly solutions applicable to various industries. These include but are not limited to conducting life cycle analyses considering green ammonia, optimization of the independency level for the decomposition system, and integrating it with various components such as dual‐fuel engines, hydrogen purification, solar energy, and fuel cells.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.175

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0030.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.344
Teacher spread0.321 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2024
Admission routes1
Has abstractyes

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