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Wood terpenes as bio-based monomers in latex for sustainable coatings

2024· article· en· W4401074141 on OpenAlexaff
Maylis Carrère, Stéphane Beaupré, Yvan Ecochard, Véronic Landry

Bibliographic record

VenueBioResources · 2024
Typearticle
Languageen
FieldEngineering
TopicLignin and Wood Chemistry
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsPetrochemicalTerpeneMaterials scienceRaw materialMonomerEconomic shortageCoatingPyrolysisThermogravimetric analysisChemical engineeringPulp and paper industryOrganic chemistryComposite materialChemistryPolymer

Abstract

fetched live from OpenAlex

Recent global market disruptions, including the COVID-19 crisis, inflation, and oil crises, have highlighted the need for industries to reduce dependence on petrochemicals. However, the coating industry remains reliant on petrochemicals due to a lack of knowledge about local and sustainable alternatives. This study explored the potential of wood extractives as precursors for producing high-quality wood coatings. Terpenes were modified through acrylation, and bio-based latexes were synthesized from these modified terpenes. Analysis showed that all tested latexes had conversion levels above 88.5%. The bio-based films were characterized, and their transparency, measured by ultraviolet-visible spectroscopy, exceeded 80%. The good incorporation of bio-based monomers in the latex films was confirmed by thermogravimetric analysis and pyrolysis-gas chromatography-mass spectrometry. Comparative analysis between bio-based and conventional latexes showed equivalent results in particle size, molecular weight, glass transition temperature, and minimum film formation temperature. However, bio-based films exhibited lower hardness. The study suggests that using monomers derived from wood extractives offers a viable alternative to petrochemicals, utilizing abundant forest residues. This approach could address raw material shortages and help make the coatings industry more sustainable by reducing its reliance on petrochemicals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.094
Threshold uncertainty score0.455

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.211
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2024
Admission routes1
Has abstractyes

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