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Coprocessing Hydrothermal Liquefaction Biocrude from Algae with Vacuum Gas Oil Using Hydrotreating

2024· article· en· W4401210581 on OpenAlexafffund
Anton Alvarez‐Majmutov, Sandeep Badoga, D.P. Singh, Patrick J. McGinn, Rafał Gieleciak, Jinwen Chen

Bibliographic record

VenueEnergy & Fuels · 2024
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsNational Research Council CanadaNatural Resources Canada
FundersOffice of Energy Research and DevelopmentNatural Resources Canada
KeywordsHydrothermal liquefactionHydrodesulfurizationAlgaeLiquefactionEnvironmental scienceVacuum distillationFuel oilPetroleumHydrothermal circulationWaste managementChemistryPulp and paper industryPetroleum engineeringChemical engineeringBiofuelCatalysisGeologyDistillationOrganic chemistryEngineeringBotanyBiology

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide In this study, we investigate the effects of coprocessing algae biocrude with petroleum in hydrotreating units. Algae biocrudes are characterized by being rich in oxygen and nitrogen components, which may pose challenges for refinery catalysts and operations. The studied biocrude was produced from a marine eustigmatophyte microalga in a hydrothermal liquefaction pilot plant and afterward it was distilled to remove excess water and high-boiling material. Coprocessing experiments were carried out in a continuous hydroprocessing pilot plant using vacuum gas oil (VGO) as the petroleum feed. The tests sought to examine different coprocessing ratios (2.5, 5, and 10 vol % biocrude in VGO) relative to baseline operation with pure VGO, as well as to determine the optimum temperature to achieve certain levels of sulfur (<300 wppm) and nitrogen (<100 wppm) removal for a given feed blend. There was a gradual decline in desulfurization activity relative to the baseline level as the coprocessing ratio increased. This unwanted effect was countered by raising reactor temperature between 2 and 6 °C over the 380 °C baseline temperature for pure VGO. Denitrogenation of the biocrude blends was achieved with ease, indicating that the nitrogen components in the biocrude distillate were mostly nonrefractory. There was no evidence to suggest that coprocessing the biocrude blends accelerated catalyst deactivation. Hydrogen consumption grew to some extent, particularly at the highest coprocessing ratio. The coprocessed products were in general less dense, had higher hydrogen content, and were richer in n -paraffins compared to the one from VGO. Biogenic carbon was found to be preserved in the liquid products at coprocessing ratios of 5% and below, whereas at a 10% ratio apparently, there were losses to gas products.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.134
Threshold uncertainty score0.833

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.218
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2024
Admission routes2
Has abstractyes

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