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Record W4401434587 · doi:10.1002/cjce.25432

Selective adsorption of aromatic sulfonic acid from wastewater using a surface imprinted polymer: H‐acid as a representative contaminant

2024· article· en· W4401434587 on OpenAlexvenueno aff
Jiaqi Yao, Yue Sun, Yan Liu, Yingpeng Gu, Weisheng Zheng

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsnot available
FundersNational Natural Science Foundation of China
KeywordsAdsorptionSulfonic acidChemistrySelectivityWastewaterPolymerSalt (chemistry)Selective adsorptionMolecularly imprinted polymerElutionDistilled waterPhthalic acidAcid dyeChromatographyNuclear chemistryOrganic chemistryCatalysisDyeing

Abstract

fetched live from OpenAlex

Abstract Aromatic sulfonic acids (ASAs) play a pivotal role as essential intermediates in numerous industrial manufacturing, while a large amount wastewater with various ASAs and high concentration of inorganic salts is subsequently generated. The effective separation and removal of ASAs from wastewater is challenging due to their complex chemical composition and the limited selectivity of common adsorbents. Herein, a novel surface imprinted polymer (H‐SIP) with high selectivity and excellent salt resistance was designed with PEI/Cl‐PS‐DVB as the carrier and 1‐amino‐8‐naphthol‐3,6‐disulfonic acid (H‐acid) as the target pollutant. Compared to non‐imprinted polymer (NIP), H‐SIP exhibited superior salt resistance in the presence of Na 2 SO 4 concentration ranging from 20 to 80 mg/L. The relative selectivity coefficients determined in the binary‐solutes experiments proved that H‐SIP demonstrated favourable selectivity towards H‐acid in binary systems of H‐acid/T‐acid or H‐acid/2‐NSA. Moreover, H‐SIP could effectively treat the simulated complex wastewater within 24 bed volume (BV) in the column adsorption, and the desorption rate exceeded 90% when eluted by NaOH solution and distilled water, respectively. Therefore, these results confirmed that surface imprinting technique was a promising method for effectively and selectively removal of ASA wastewater in the application.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.025
Threshold uncertainty score0.699

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.252
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2024
Admission routes1
Has abstractyes

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