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Record W4401973293 · doi:10.1038/s43246-024-00594-1

Static magnetic order with strong quantum fluctuations in spin-1/2 honeycomb magnet Na2Co2TeO6

2024· article· en· W4401973293 on OpenAlexafffund
Jinlong Jiao, Xiyang Li, Gaoting Lin, Mingfang Shu, Wei Xu, O. Zaharko, T. Shiroka, Tao Hong, А. И. Колесников, Guochu Deng, S. R. Dunsiger, M. C. Aronson, Haidong Zhou, Xiaoqun Wang, Tian Shang, Jie Ma

Bibliographic record

VenueCommunications Materials · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsSimon Fraser UniversityTRIUMFUniversity of British Columbia
FundersDivision of Materials ResearchStewart Blusson Quantum Matter Institute, University of British ColumbiaNatural Sciences and Engineering Research Council of CanadaOffice of ScienceCentre Scientifique et Technique du BâtimentSimon Fraser UniversityPaul Scherrer InstitutEast China Normal UniversityCanada First Research Excellence FundNatural Science Foundation of ChongqingHuazhong University of Science and TechnologyOak Ridge National LaboratoryNational Natural Science Foundation of ChinaU.S. Department of EnergyMinistry of Education, IndiaAustralian Nuclear Science and Technology OrganisationShanghai Jiao Tong UniversityZhejiang UniversityNational Science FoundationTRIUMFNatural Science Foundation of ShanghaiNational Key Research and Development Program of ChinaEidgenössische Technische Hochschule Zürich
KeywordsMuon spin spectroscopyCondensed matter physicsQuantum spin liquidPhysicsAntiferromagnetismFrustrationSpin (aerodynamics)Neutron scatteringQuantum fluctuationGround stateSpin waveQuantumScatteringQuantum mechanicsSpin polarizationFerromagnetismElectron

Abstract

fetched live from OpenAlex

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev interactions typically promote a zigzag antiferromagnetic order in the d-orbital transition-metal compounds. Here, by combining neutron scattering with muon-spin rotation and relaxation techniques, we provide mechanism insights into the exotic properties of Na2Co2TeO6, a candidate material of the Kitaev model. Below TN, the zero-field muon-spin relaxation rate becomes almost constant (~0.45 μs−1). We attribute this temperature-independent relaxation rate to the strong quantum fluctuations, as well as to the frustrated Kitaev interactions. As the magnetic field increases, neutron scattering data indicate a broader spin-wave excitation at the K-point. Therefore, quantum fluctuations seem not only robust but are even enhanced by the applied magnetic field. Our findings provide valuable hints for understanding the onset of the quantum-spin-liquid state in Kitaev materials. Na2Co2TeO6 is a candidate Kitaev spin-liquid, but the nature of its ground state remains controversial, as spurious non-Kitaev exchange interactions promote magnetic ordering. Here, neutron scattering and muon-spin rotation experiments indicate the presence of strong quantum fluctuations in the ground state, giving rise to a multi-domain zigzag antiferromagnetic order.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.297
Teacher spread0.280 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2024
Admission routes2
Has abstractyes

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