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Record W4402424613 · doi:10.1016/j.chemgeo.2024.122392

Robust methods, tricky materials: Challenges in dating high common-Pb perovskite from Cretaceous Brazilian kimberlites

2024· article· en· W4402424613 on OpenAlexafffund
Rogério Guitarrari Azzone, D. Graham Pearson, C. K. Sarkar, Lina Cetina, Luanna Chmyz, Yaqin Luo, Excelso Ruberti, Vincenza Guarino, Izaac Cabral-Neto

Bibliographic record

VenueChemical Geology · 2024
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeological and Geochemical Analysis
Canadian institutionsUniversity of Alberta
FundersConselho Nacional de Desenvolvimento Científico e TecnológicoFundação de Amparo à Pesquisa do Estado de São PauloUniversity of Alberta
KeywordsKimberliteGeologyCretaceousGeochemistryPaleontologyPerovskite (structure)Earth scienceMantle (geology)Chemical engineering

Abstract

fetched live from OpenAlex

Kimberlites and related rocks are the focus of research and exploration in the Alto Paranaiba Igneous Province (APIP; Brazil) due to their potential correlation with adjacent diamond fields. New U-Pb perovskite ages were obtained using recommended protocols for error propagation and data interpretation. Despite the utility of perovskites for dating, their incorporation of significant common-Pb (common-Pb of new APIP data: 52–84 % for in situ analyses, 75–95 % for TIMS concentrate analyses) limits the age resolution of this dating approach. Consequently, the APIP U-Pb ages neither confirm nor discredit previously proposed geodynamic models that invoke age progression or distinct magmatic episodes. Comparing the new ID-TIMS and LA-ICP-MS ages of the same intrusions, the LA-ICP-MS data have lower uncertainties, largely due to accessing a greater spread in common-Pb, improving regressions, and tend to yield older ages. For perovskite grains collected from weathering profiles , we found evidence of Pb-loss. This process leads to higher uncertainties in individual analyses, increased data scatter, and consequently higher uncertainties in age estimates. For fresh samples with different degrees of crustal contamination from a single intrusion, we found an indication of some variability in 207 Pb/ 206 Pb and 238 U/ 206 Pb ratios of the perovskite data, with a tendency towards older ages for more contaminated sample. For almost fresh intrusions with geochemically and isotopically similar mantle sources , related to the same event and in a close geographic area , we prefer to use a unique local 207 Pb/ 206 Pb ratio as anchoring for each Tera-Wasserburg plot. This approach is particularly preferred when perovskite data of an intrusion are too clustered and the 207 Pb/ 206 Pb ratio from the unanchored T-W differs from that predicted from theoretical Pb-isotope evolution model. Despite the high-common Pb in APIP perovskite crystals, our new data using these strategies clearly indicate that APIP magmatism is restricted to the Cretaceous, with most cases crystallized in Upper Cretaceous , but some from Early Cretaceous , such as the diamondiferous occurrence of Catalão-1b (120.6 ± 6.7 Ma). Different triggers of APIP magmatism are related to both episodes, mainly attributed to supercontinent break-up stages.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Other design · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.621
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0380.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.048
GPT teacher head0.265
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designOther design
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2024
Admission routes2
Has abstractyes

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