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Record W4402521167 · doi:10.5194/acp-24-10159-2024

Biomass burning CO emissions: exploring insights through TROPOMI-derived emissions and emission coefficients

2024· article· en· W4402521167 on OpenAlexaff
Debora Griffin, Jack Chen, Kerry Anderson, Paul A. Makar, C. A. McLinden, Enrico Dammers, Andre Fogal

Bibliographic record

VenueAtmospheric chemistry and physics · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsUniversity of SaskatchewanUniversity of WaterlooNational Institute for NanotechnologyEnvironment and Climate Change Canada
FundersEuropean CommissionNASA HeadquartersNetherlands Space OfficeEuropean Space AgencyNational Aeronautics and Space Administration
KeywordsEnvironmental scienceSCIAMACHYEmission inventoryTrace gasAtmospheric sciencesSatelliteBiomass burningTroposphereCombustionGreenhouse gasNorthern HemisphereAir quality indexBiomass (ecology)MeteorologyAerosolChemistryGeography

Abstract

fetched live from OpenAlex

Emissions from biomass burning are a significant source of air pollution, which can adversely impact air quality and ecosystems thousands of kilometres downwind. These emissions can be estimated by a bottom-up approach that relies on fuel consumed and standardized emission factors. Emissions are also commonly derived with a top-down approach, using satellite-observed fire radiative power (FRP) as a proxy for fuel consumption. Biomass burning emissions can also be estimated directly from satellite trace gas observations, including carbon monoxide (CO). Here, we explore the potential of satellite-derived CO emission rates from biomass burning and provide new insights into the understanding of satellite-derived fire CO emissions globally, with respect to differences in regions and vegetation type. Specifically, we use the TROPOMI (Tropospheric Monitoring Instrument) high-spatial-resolution satellite datasets to derive burning CO emissions directly for individual fires between 2019 and 2021 globally. Using synthetic data (with known emissions), we show that the direct emission estimate methodology has a 34 % uncertainty for deriving CO emissions (and a total uncertainty of 44 % including wind and CO column uncertainty). From the TROPOMI-derived CO emissions, we derive biome-specific emission coefficients (emissions relative to FRP) by combining the direct emission estimates and the satellite-observed FRP from the Moderate Resolution Imaging Spectrometer (MODIS). These emission coefficients are used to establish annual top-down CO emission inventories from biomass burning, showing that Southern Hemisphere Africa has the highest CO biomass burning emissions (over 25 % of global total of 300–390 Mt(CO) yr −1 between 2003–2021), and almost 25 % of global CO biomass burning emissions are from broadleaved evergreen tree fires. A comprehensive comparison between direct estimates, top-down and bottom-up approaches, provides insight into the strengths and weaknesses of each method: FINN2.5 has higher CO emissions, by a factor between 2 and 5, than all other inventories assessed in this study. Trends over the past 2 decades are examined for different regions around the globe, showing that global CO biomass burning emissions have, on the whole, decreased (by 5.1 to 8.7 Mt(CO) yr −1 ), where some regions experience increased and others decreased emissions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.040
Threshold uncertainty score0.079

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.231
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2024
Admission routes1
Has abstractyes

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