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Record W4403094251 · doi:10.1088/1361-6528/ad82f1

Enhancement of photoresponse for InGaAs infrared photodetectors using plasmonic WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> /Cs<sub>y</sub>WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> nanocrystals

2024· article· en· W4403094251 on OpenAlex
Zach D. Merino, Gyorgy Jaics, Andrew W. M. Jordan, Arjun Shetty, Penghui Yin, Man Chun Tam, Xinning Wang, Z. R. Wasilewski, Pavle V. Radovanovic, Jonathan Baugh

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueNanotechnology · 2024
Typearticle
Languageen
FieldMaterials Science
TopicGa2O3 and related materials
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaCanada First Research Excellence FundCanada Foundation for Innovation
KeywordsMaterials sciencePhotodetectorInfraredPlasmonOptoelectronicsNanocrystalNanotechnologyOptics

Abstract

fetched live from OpenAlex

Abstract Fast and accurate detection of light in the near-infrared (NIR) spectral range plays a crucial role in modern society, from alleviating speed and capacity bottlenecks in optical communications to enhancing the control and safety of autonomous vehicles through NIR imaging systems. Several technological platforms are currently under investigation to improve NIR photodetection, aiming to surpass the performance of established III–V semiconductor p-i-n (PIN) junction technology. These platforms include in situ -grown inorganic nanocrystals (NCs) and nanowire arrays, as well as hybrid organic–inorganic materials such as graphene-perovskite heterostructures. However, challenges remain in NC and nanowire growth, large-area fabrication of high-quality 2D materials, and the fabrication of devices for practical applications. Here, we explore the potential for tailored semiconductor NCs to enhance the responsivity of planar metal–semiconductor–metal (MSM) photodetectors. MSM technology offers ease of fabrication and fast response times compared to PIN detectors. We observe enhancement of the optical-to-electric conversion efficiency by up to a factor of ∼2.5 through the application of plasmonically-active semiconductor nanorods and NCs. We present a protocol for synthesizing and rapidly testing the performance of non-stoichiometric tungsten oxide (WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> ) nanorods and cesium-doped tungsten oxide (Cs y WO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> <mml:mi>x</mml:mi> </mml:mrow> </mml:msub> </mml:mrow> </mml:math> ) hexagonal nanoprisms prepared in colloidal suspensions and drop-cast onto photodetector surfaces. The results demonstrate the potential for a cost-effective and scalable method exploiting tailored NCs to improve the performance of NIR optoelectronic devices.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.008
metaresearch head score (Gemma)0.006
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Open science, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity, Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.678
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0080.006
Meta-epidemiology (narrow)0.0040.007
Meta-epidemiology (broad)0.0020.006
Bibliometrics0.0030.005
Science and technology studies0.0050.007
Scholarly communication0.0050.005
Open science0.0080.008
Research integrity0.0110.006
Insufficient payload (model declined to judge)0.4410.007

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.243
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it