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Record W4403144312 · doi:10.1111/jace.20181

Effect of BaO on viscosity and structure of B <sub>2</sub> O <sub>3</sub> –SiO <sub>2</sub> –Al <sub>2</sub> O <sub>3</sub> –Na <sub>2</sub> O–BaO glass lubricant

2024· article· en· W4403144312 on OpenAlexaff
Lei Cui, Peiyuan Ni, Wei Lv, Ying Li

Bibliographic record

VenueJournal of the American Ceramic Society · 2024
Typearticle
Languageen
FieldEngineering
TopicMetallic Glasses and Amorphous Alloys
Canadian institutionsUniversity of Toronto
FundersFundamental Research Funds for the Central UniversitiesNational Natural Science Foundation of China
KeywordsMaterials scienceMineralogyCrystallographyChemistry

Abstract

fetched live from OpenAlex

Abstract Glass lubricant with a suitable viscosity is critical for the efficient production of high‐quality titanium alloy in hot extrusion process. In this study, a new glass lubricant, (30.93‐0.309 x )B 2 O 3 ‐(48.45‐0.485 x )SiO 2 ‐(7.22‐0.072 x )Al 2 O 3 ‐(13.4‐0.134 x )Na 2 O‐ x BaO (BSANB), was proposed for titanium alloy hot extrusion. The effect of BaO content varying from 0 wt.% to 15 wt.% on its viscosity was investigated, and the mechanism of viscosity change was clarified through melt structure analysis by using molecular dynamics (MD) simulation, X‐ray photoelectron spectroscopy (XPS), and Raman spectroscopy. The glass viscosity was measured in the temperature range of 950°C to 1100°C, and the atomic self‐diffusion coefficient of the glass melt was calculated. The results demonstrated that the BaO content has a significant influence on the viscosity of the BSANB glass at the hot extrusion temperature range. The viscosity value at 950°C was decreased by 52.87%, from 103.5 Pa·s to 48.8 Pa·s, when BaO content was increased from 0 wt.% to 15 wt.%. MD simulation results of the BSANB glass show that the self‐diffusion coefficient of Si atoms was lower than that of Al and B atoms, indicating that Si‐O bonds were more stable in the melt. The diffusion coefficient of Si atom was directly related to the rheological behavior of the melt, which can be reflected by the melt viscosity. The results of MD simulation, XPS and Raman spectral fitting at 950°C showed an increase in the amounts of Q 1 , Q 0 and [BO 4 ], while the amounts of Q 2 , Q 3 , Q 4 and [AlO 4 ] were decreased when BaO content was increased from 0 wt.% to 15 wt.%. This demonstrated that the melt network was depolymerized with an increased BaO content, which determined the melt viscosity change. In addition, the mechanism responsible for glass viscosity reduction due to temperature increase was also discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity
Consensus categoriesMeta-epidemiology (narrow), Research integrity
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.070
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.001
Meta-epidemiology (narrow)0.0040.003
Meta-epidemiology (broad)0.0060.005
Bibliometrics0.0010.004
Science and technology studies0.0010.002
Scholarly communication0.0010.001
Open science0.0030.001
Research integrity0.0010.006
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.212
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2024
Admission routes1
Has abstractyes

Explore more

Same venueJournal of the American Ceramic SocietySame topicMetallic Glasses and Amorphous AlloysFrench-language works237,207