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Record W4403491200 · doi:10.1002/cjce.25528

A study on the kinetics of the gas–liquid reaction between nitric oxide and [Fe( <scp>II</scp> ) <scp>NTA</scp> ] <sup>−</sup>

2024· article· en· W4403491200 on OpenAlexvenueno aff
Ning Ma, Dong Li, Xiang‐li Long

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsnot available
Fundersnot available
KeywordsKineticsNitric oxideChemistryChemical kineticsNitric acidNuclear chemistryChemical engineeringInorganic chemistryOrganic chemistryPhysicsEngineering

Abstract

fetched live from OpenAlex

Abstract Iron nitrilotriacetic acid ([Fe(II)NTA] − ) solution is able to absorb NO from flue gases. In this study, the kinetics of the gas–liquid reaction between NO and [Fe(II)NTA] − has been determined using a double stirred cell. The study indicates that the reaction between NO and [Fe(II)NTA] − is turned into gas film controlling as the [Fe(II)NTA] − concentration is over 0.03 mol L −1 . The reaction rate between NO and [Fe(II)NTA] − is in proportion to the inlet nitric oxide concentration. 50°C is considered to be the best temperature for [Fe(II)NTA] − solution absorbing nitric oxide. The reaction rate between NO and [Fe(II)NTA] − decreases as pH drops below 5.5. The negative effect of pH may be reduced as the [Fe(II)NTA] − concentration increases. The reaction rate between NO and [Fe(II)NTA] − varies little in the pH range from 5.5 to 8.0. The kinetic equation for the gas–liquid reaction between NO and [Fe(II)NTA] − under the controlling of both liquid film and gas film has been obtained as follows: The activation energy E a for the gas–liquid reaction between NO and [Fe(II)NTA] − is 13.06 KJ/mol. stands for the rate of chemisorptions, mol/(m 2 · s); for the NO concentration in the interface, mol L −1 ; and for [Fe(II)NTA] − concentration in the liquid, mol L −1 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.219
Teacher spread0.205 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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