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Modelling the black and brown carbon absorption and their radiative impact: the June 2023 intense Canadian boreal wildfires case study

2024· preprint· en· W4403634788 on OpenAlexaboutno aff
Paolo Tuccella, Ludovico Di Antonio, Andrea Di Muzio, Colaiuda Valentina, Laurent Menut, Giovanni Pitari, Edoardo Raparelli

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsnot available
Fundersnot available
KeywordsArcticEnvironmental scienceBorealCarbon blackAtmospheric sciencesTaigaRadiative transferAbsorption (acoustics)ClimatologyClimate changeThe arcticCarbon fibersClimate modelGeographyPhysicsOceanographyChemistryMaterials scienceGeologyForestryArchaeology

Abstract

fetched live from OpenAlex

Black carbon (BC) and brown carbon (BrC) are light-absorbing aerosols with significant climate impacts, but their absorption properties and direct radiative effect (DRE) remain uncertain. We simulated BC and BrC absorption during the intense Canadian boreal wildfires in June 2023 using an enhanced version of CHIMERE model. The study focused on a domain extending from North America to Eastern Europe, including a significant portion of the Arctic up to 85°N. The enhanced model includes an updated treatment for the BC absorption enhancement and a BrC ageing scheme accounting for both browning and blanching through oxidation. When compared to observations, the updated model accurately captured aerosol optical depth (AOD) at multiple wavelengths, both near the wildfires and during transoceanic transport to Europe. Improvements were observed in the simulation of absorbing aerosol optical depth (AAOD) compared to the control model. The all-sky regional direct radiative effect (DRE) for June 2023 attributed to the intense Canadian wildfires, was reduced from -2.1 W/m² in the control model to -1.9 W/m² (-2.0/-1.8 W/m², ±5%), in the enhanced model, indicating an additional warming effect of +0.2 W/m² (about +10%) due to advanced schemes used for the BC and BrC absorption. The results indicate the importance of an accurate simulation of aerosol absorption in regional climate predictions, especially during large-scale biomass burning events. They also suggest that traditional models could overestimate the cooling effect of boreal wildfires, highlighting the need for improvement of aerosol parameterization to better predict the DRE and develop effective mitigation strategies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.104
Threshold uncertainty score0.209

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0020.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.000
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.229
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes1
Has abstractyes

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