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Record W4403932194 · doi:10.1016/j.epsl.2024.119097

The sulfur isotopic composition of Cenozoic pyrite is affected by methane content and depositional environment

2024· article· en· W4403932194 on OpenAlexaff
Charlotte Spruzen, Harold J. Bradbury, Emma Kast, Alexandra V. Turchyn

Bibliographic record

VenueEarth and Planetary Science Letters · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicMethane Hydrates and Related Phenomena
Canadian institutionsUniversity of British ColumbiaMcGill University
FundersUniversity of CambridgeNatural Environment Research CouncilSight Research UK
KeywordsSedimentary depositional environmentGeologyPyriteCenozoicGeochemistryMethaneSulfurComposition (language)MineralogyPaleontologyStructural basinChemistry

Abstract

fetched live from OpenAlex

• Outcrop δ 34 S pyr is dependent on water depth and lithology. • Sediment δ 34 S pyr is dependent on methane content, sedimentation rate and lithology. • Modern ‘superheavy’ pyrite forms in sediment with high methane concentrations. • There are no clear trends in average δ 34 S pyr over the past 165 million years. The sulfur isotopic composition of pyrite (δ 34 S pyr ) is often used to reconstruct ancient geobiological processes, but recent studies have shown that δ 34 S pyr is strongly dependent on local sedimentary environmental conditions. Here we present a global compilation of >3700 published pyrite sulfur isotopic compositions from the past 165 million years, from outcrop as well as marine sediment cores. We show that sediment core δ 34 S pyr has a statistically significant relationship with methane content, sedimentation rate, lithology, and proximity from shore, while outcrop δ 34 S pyr has distinct distributions depending on categories of depositional water depth and lithology. There are no obvious trends in the average δ 34 S pyr from the late Mesozoic to the present, although we suggest that this temporal record is affected by the inherent bias of data compilation. Our study further emphasizes the importance of considering sedimentology and stratigraphic context when using the sulfur isotopic composition of pyrite to infer global environmental changes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.876
Threshold uncertainty score0.341

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.174
Teacher spread0.167 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2024
Admission routes1
Has abstractyes

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