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Record W4403941788 · doi:10.1021/acssuschemeng.4c06833

Paper-Supported Sodium Alginate Composite Separator Prepared by Polymer-Assisted Phase Separation for Lithium Ion Batteries

2024· article· en· W4403941788 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2024
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsUniversity of Alberta
FundersNational Natural Science Foundation of China
KeywordsSeparator (oil production)Composite numberIonLithium (medication)Materials sciencePolymerChemical engineeringSodiumCompatibility (geochemistry)Sodium alginateInorganic chemistryChemistryOrganic chemistryComposite materialMetallurgy

Abstract

fetched live from OpenAlex

Ecofriendly and renewable properties are highly desirable for separators of lithium batteries, apart from the notorious safety issues. As a natural polysaccharide material, sodium alginate (SA) has outstanding biodegradability and biocompatibility and has usually been used for the binder of electrodes due to its high ionic conductivity. Herein, SA porous separators were initially prepared by a facile polymer-assisted phase separation in which polyethylene glycol (PEG) and acetonitrile acted as a pore-forming agent and an extraction solvent, respectively. The influence of PEG content on the pore formation was systematically investigated, and the uniform and continuous pore structures were successfully realized at the PEG content of 200–500 wt %. Additionally, the cellulose-based paper support (KP) and poly(vinylidene fluoride- co -hexafluoropropylene) porous coating (PVH) were adopted for the decent mechanical integrity of SA porous membranes. The prepared SA composite separators showed excellent thermal dimensional stability, high porosity, and good electrolyte wettability. Moreover, the polar features of SA endowed the composite separators with high ionic conductivity (4.8 mS cm –1 ) and lithium ion transference number (0.62). The strong depression capacity of lithium dendrites and a comparable electrochemical performance were also observed for the SA-based separators compared with the pure KP and commercial polyolefin separators.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.322
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.257
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it