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Record W4404029413 · doi:10.1002/cjce.25537

Overcoming clay structure challenges in lithium recovery from boron waste using high‐temperature pressure acid leaching

2024· article· en· W4404029413 on OpenAlex
Nebil Younes, M. Deniz Turan, Mehmet Erdem

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2024
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsnot available
FundersFirat University Scientific Research Projects Management Unit
KeywordsBoronLeaching (pedology)Materials scienceWaste managementLithium (medication)Lithium borateEnvironmental scienceChemical engineeringChemistrySoil scienceBorate glassEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Boron mines contain significant amounts of lithium along with boron. After boron is extracted, lithium remains in the waste, which has a carbonate‐hosted clay‐type structure, along with other impurities. The scarcity of lithium resources and the increasing need for lithium worldwide make such resources economically important. Although the best hydrometallurgical method for the recovery of lithium trapped within the clay‐structured mineral resources is roasting with chemicals to disrupt the clay structure and acid leaching, the process is quite difficult and costly due to the high energy and chemical addition requirements. To overcome this challenge, this study proposed a high‐temperature–pressure sulphuric acid leaching process to recover lithium from the boron waste. Under the optimized conditions (liquid/solid ratio: 10, acid concentration: 1 M, temperature: 150°C, and contact time: 120 min), 100% of lithium was leached. The leaching mechanism was determined through mineral characterization (X‐ray diffractometry [XRD], X‐ray fluorescence spectrophotometer [XRF], scanning electron microscopy–energy‐dispersive X‐ray spectroscopy [SEM–EDX], Mastersizer), and a shrinking core heterogeneous kinetics model. It was found that high‐temperature–pressure sulphuric acid leaching disrupted clay structure and promoted the leaching of lithium, the leaching kinetics fit the shrinking core heterogeneous kinetics model, and was controlled by a dual mechanism with ash diffusion and chemical reactions on the particle surface. The reaction rate constants increased with increasing temperature, and the activation energy was found to be 32.17 kJ/mol.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.218
Threshold uncertainty score0.605

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.211
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it