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Record W4404090398 · doi:10.1021/acs.estlett.4c00757

Quaternary Ammonium Compounds in Paired Samples of Blood and Indoor Dust from the United States

2024· article· en· W4404090398 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueEnvironmental Science & Technology Letters · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicEnvironmental Chemistry and Analysis
Canadian institutionsARC Resources (Canada)
FundersIndiana Clinical and Translational Sciences InstituteNational Natural Science Foundation of ChinaIndiana University
KeywordsQuaternaryAmmoniumEnvironmental chemistryEnvironmental scienceChemistryGeologyPaleontologyOrganic chemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Previous studies of quaternary ammonium compounds (QACs) in the indoor environment have reported widespread presence of QAC in indoor dust. However, there are limited data on the contribution of dust ingestion to the QAC body burden. In this study, 18 QACs (6 benzylalkyldimethylammonium compounds [BACs], 6 dialkyldimethylammonium compounds [DADMACs], and 6 alkyltrimethylammonium compounds [ATMACs]) were analyzed in 81 paired samples of blood serum and dust collected in Indiana, United States. QACs were detected in 51–100% of the dust samples with the total QAC concentrations (∑QAC) ranging from 0.613 to 427 μg/g (median 56.9 μg/g). In contrast to dust samples, QACs were detected less frequently in blood serum with a median ∑QAC concentration of 3.66 ng/mL. The relative source contribution (RSC) of dust ingestion to serum levels was calculated using the PROTEX (PROduction-To-EXposure) model and was estimated as less than 1%, suggesting that hand-to-mouth contact, dietary intake, or inhalation could be more important exposure routes than dust ingestion. This is the first study to simultaneously measure QAC concentrations in indoor dust and blood, providing comprehensive assessment of the role of dust ingestion in QAC human exposure.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.037
Threshold uncertainty score0.996

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.006
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.190
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it