MétaCan
Menu
Back to cohort
Record W4404327916 · doi:10.1002/smtd.202401179

Highly Active NiRu/C Cathode Catalyst Synthesized by Displacement Reaction for Anion Exchange Membrane Water Electrolysis

2024· article· en· W4404327916 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueSmall Methods · 2024
Typearticle
Languageen
FieldEnergy
TopicElectrocatalysts for Energy Conversion
Canadian institutionsnot available
FundersNational Research Council Canada
KeywordsCatalysisElectrolysisGalvanic cellCathodeChemical engineeringAnodeMaterials scienceElectrolysis of waterInorganic chemistryHydrogenHydrogen productionMembraneIon exchangeElectrolytic cellChemistryElectrolyteIonMetallurgyElectrodePhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Anion exchange membrane water electrolysis (AEMWE) is highly promising for cost‐effective green hydrogen production due to its basic operating conditions facilitating the use of non‐noble catalysts. While non‐noble Ni/Fe‐based catalysts are utilized at the anode, its cathode catalyst still requires precious Pt. Due to the high cost of Pt and the sluggish hydrogen evolution reaction (HER) at the cathode in basic conditions, developing alternative catalysts to replace Pt is highly important. Here, a synthesis procedure for a Ru‐based catalyst is reported and its high activity toward the HER in alkaline media is demonstrated in both half‐cell and single‐cell tests. The catalyst is synthesized in a two‐step approach. A highly dispersed Ni catalyst is prepared on carbon support in the first step. In the second step, Ru is deposited on its surface using a galvanic displacement reaction. The uniqueness of this method is that Ru is deposited over the entire electrically conductive surface, resulting in an isotropic and homogeneous Ru distribution within the catalyst powder. It is demonstrated that this material remarkably outperforms state‐of‐the‐art Pt/C catalysts in half‐cell and single‐cell tests. The single cell only requires 1.73 V at 1 A cm −2 with an overall PGM content of 0.05 mg cm −2 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.436
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.298
Teacher spread0.280 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it