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Record W4404366540 · doi:10.1002/ejlt.202400081

Effect of Fat Composition on Allylic Proton Transverse Relaxation and J‐Coupling Evolution at 9.4 T

2024· article· en· W4404366540 on OpenAlexaff
Nathaniel Bly, Adam Carscadden, Alexander Dehod, Anthony G. Tessier, Catherine J. Field, Atiyah Yahya

Bibliographic record

VenueEuropean Journal of Lipid Science and Technology · 2024
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsAllylic rearrangementComposition (language)Coupling (piping)Transverse planeProtonRelaxation (psychology)ChemistryChemical physicsPhysicsMaterials scienceNuclear physicsOrganic chemistryBiologyComposite materialAnatomyCatalysis

Abstract

fetched live from OpenAlex

Abstract Transverse ( T 2 ) relaxation and J‐coupling evolution of oleic, linoleic, and linolenic acid allylic protons are investigated at 9.4 T as an indirect means of assessing fat composition. We hypothesize that the relative proximity of one allylic proton group to the methyl end of the fatty acid impacts the measures. A Point RESolved Spectroscopy (PRESS) sequence was used for apparent (includes J‐coupling effects) T 2 estimation. Spectra were acquired from oleic, linoleic, and linolenic acid, from edible oils, and from intraperitoneal adipose tissue of two groups of mice ( n = 4 per group) randomized to a high or low ω‐3 diet. Apparent T 2 values of 62, 106, and 220 ms were obtained for oleic, linoleic, and linolenic acid allylic protons, respectively. For oils containing negligible linolenic acid, apparent T 2 values correlated with linoleic acid contribution to total unsaturation ( R 2 = 1). For oils containing linolenic acid, a correlation with linolenic acid contribution to total unsaturation was found ( R 2 = 0.91). In animal experiments, the mean allylic apparent T 2 in the group fed the high ω‐3 diet was 72.3 ms compared to 66.1 ms measured from the low ω‐3 diet group. Signal yield with an echo time (TE) of 130 ms results in an inverse correlation with relative linolenic acid content ( R 2 = 0.99) for the oils.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.493
Threshold uncertainty score0.200

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.213
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

Explore more

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