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Record W4404679206 · doi:10.1002/dta.3832

Doping Control Analysis of Total Carbon Dioxide (TCO<sub>2</sub>) in Equine Plasma by Headspace Gas Chromatography–Mass Spectrometry (HS‐GC/MS)

2024· article· en· W4404679206 on OpenAlexaffabout
Karen Y. Kwok, Wai-Him Kwok, Terence S. M. Wan, Lydia Brooks, Marie‐Agnès Popot, Murielle Jaubert, Ludovic Bailly‐Chouriberry, Brendan Heffron, Bob McKenzie, Naomi Selvadurai, David Batty, Bobby Gray, Stefania Ragazzoni, Mariani Claudio, Emmie N. M. Ho

Bibliographic record

VenueDrug Testing and Analysis · 2024
Typearticle
Languageen
FieldMedicine
TopicRenal function and acid-base balance
Canadian institutionsAdvantage Forensics (Canada)Canadian Space Agency
Fundersnot available
KeywordsMass spectrometryGas chromatography–mass spectrometryCarbon dioxideChemistryChromatographyGas chromatographyAnalytical Chemistry (journal)Organic chemistry

Abstract

fetched live from OpenAlex

ABSTRACT The use of alkalinising agents prior to racing for manipulating performance in the horse has been identified since the 1990s. To mitigate the risk, an international threshold for available carbon dioxide in equine plasma based on analyses using the Beckman Synchron EL ‐ISE analyser was adopted in 1994 by the International Federation of Horseracing Authorities (IFHA) and revised from 37 to 36 mM in 2004. In 2009, the technical support for the above instrument was discontinued by its manufacturer. Based on the same measurement principle (i.e., ion selective electrode), the Beckman DxC600 analyser was selected as an alternative and validated against the protocol developed by the Association of Official Racing Chemists (AORC). Recently, the DxC600 analyser is also no longer supported by Beckman. Various alternative methods for measuring total carbon dioxide (TCO 2 ) in plasma have been explored. Among these, a headspace gas chromatography–mass spectrometry (HS‐GC/MS) method was first reported by the Analytical Forensic Testing Laboratory (AFTL) in 2017. Methods based on the same measurement principle were later developed by different horseracing laboratories. With the objective of cross‐validating the new HS‐GC/MS methods and to establish an absolute (rather than instrument‐dependent or empirical) threshold, an international research collaboration was initiated among different racing laboratories. This paper describes the results of cross‐validation studies conducted in November 2019 and December 2022 using horse administration samples from Canada and France, respectively, the determination of a threshold based on population data, and some technical insights on the HS‐GC/MS methods.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.711
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0030.012
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.234
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes2
Has abstractyes

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