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Record W4404729239 · doi:10.1002/advs.202407625

Unconventional Anomalous Hall Effect Driven by Self‐Intercalation in Covalent 2D Magnet Cr<sub>2</sub>Te<sub>3</sub>

2024· article· en· W4404729239 on OpenAlexafffund
Keke He, Mengying Bian, Samuel D. Seddon, Koushik Jagadish, Andrea Mucchietto, Ren He, Erik Kirstein, Reza Asadi, Jaeil Bai, Chao Yao, Sheng Pan, Jie-Xiang Yu, Peter Milde, Chang Huai, Haolei Hui, Jiadong Zang, Renat Sabirianov, Xuemei Cheng, Guo‐Xing Miao, Hui Xing, Yu‐Tsun Shao, S. A. Crooker, Lukas M. Eng, Yanglong Hou, F. Bird, Hao Zeng

Bibliographic record

VenueAdvanced Science · 2024
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsUniversity of Waterloo
FundersBasic Energy SciencesDivision of Electrical, Communications and Cyber SystemsNational Key Research and Development Program of ChinaNatural Sciences and Engineering Research Council of CanadaDivision of Materials Sciences and EngineeringNational Natural Science Foundation of ChinaNational High Magnetic Field LaboratoryU.S. Department of EnergyDivision of Materials ResearchCanada First Research Excellence FundNational Science Foundation
KeywordsSpintronicsCondensed matter physicsHall effectMaterials scienceIntercalation (chemistry)Berry connection and curvatureHysteresisMagnetNanotechnologyChemistryMagnetic fieldPhysicsFerromagnetismInorganic chemistryGeometric phase

Abstract

fetched live from OpenAlex

Abstract Covalent 2D magnets such as Cr 2 Te 3 , which feature self‐intercalated magnetic cations located between monolayers of transition‐metal dichalcogenide material, offer a unique platform for controlling magnetic order and spin texture, enabling new potential applications for spintronic devices. Here, it is demonstrated that the unconventional anomalous Hall effect (AHE) in Cr 2 Te 3 , characterized by additional humps and dips near the coercive field in AHE hysteresis, originates from an intrinsic mechanism dictated by the self‐intercalation. This mechanism is distinctly different from previously proposed mechanisms such as topological Hall effect, or two‐channel AHE arising from spatial inhomogeneities. Crucially, multiple Weyl‐like nodes emerge in the electronic band structure due to strong spin‐orbit coupling, whose positions relative to the Fermi level is sensitively modulated by the canting angles of the self‐intercalated Cr cations. These nodes contribute strongly to the Berry curvature and AHE conductivity. This component competes with the contribution from bands that are less affected by the self‐intercalation, resulting in a sign change in AHE with temperature and the emergence of additional humps and dips. The findings provide compelling evidence for the intrinsic origin of the unconventional AHE in Cr 2 Te 3 and further establish self‐intercalation as a control knob for engineering AHE in complex magnets.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.247
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2024
Admission routes2
Has abstractyes

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