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Record W4404729942 · doi:10.1055/a-2487-4285

Entirely Biomass-Derived Hydrogel Composites for Possible Applications in Drug Delivery

2024· article· en· W4404729942 on OpenAlexafffund
Megan Marie Fitzgerald, Francesca M. Kerton

Bibliographic record

VenueSustainability & Circularity NOW · 2024
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicHydrogels: synthesis, properties, applications
Canadian institutionsMemorial University of Newfoundland
FundersDepartment of Industry, Energy and TechnologyNatural Sciences and Engineering Research Council of CanadaMemorial University of NewfoundlandCanada Foundation for Innovation
KeywordsBiomass (ecology)Drug deliveryComposite materialMaterials scienceSelf-healing hydrogelsNanotechnologyPolymer chemistryEcologyBiology

Abstract

fetched live from OpenAlex

Abstract Entirely biomass-based chitosan-alginate hydrogel composites were prepared using mussel-derived calcite. Composite hydrogel beads were prepared with 0.0, 1.0, and 2.5 wt % calcite and were characterized using IR spectroscopy, scanning electron microscopy (SEM), and thermogravimetric analysis (TGA). Diameters of beads were measured to ensure uniform preparation. The swelling behavior of beads was tested in 0.1 M HCl, 0.1 M potassium phosphate buffer, and deionized water at 37 °C. Beads containing calcite were found to have significantly less swelling ability in 0.1 M HCl and deionized water, but in 0.1 M potassium phosphate buffer, no change in swelling ability was observed for beads containing zero calcite compared with those containing calcite. Encapsulation efficiency (EE) measurements of methylene blue, as a model drug, showed that 0.0 wt % calcite beads had an EE of 80.8% and those containing calcite had lower EE: 60.7% (1.0 wt % calcite) and 71.6% (2.5 wt % calcite). Methylene blue release in a surrogate gastric environment (0.1 M HCl followed by 0.1 K buffer) showed that 0.0 wt % calcite beads had the least controlled release, whereas those containing calcite showed controlled release. Drug release results were found to be significant through a one-way ANOVA test (p < 0.05). TGA data show that SC levels in beads after placement in a surrogate gastric fluid (0.1 M HCl) are significantly reduced due to the reaction between calcite and HCl.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.260
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes2
Has abstractyes

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