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Record W4404965809 · doi:10.1021/acsestwater.4c00796

How the δ<sup>18</sup>O<sub>NO<sub>3</sub></sub> versus δ<sup>15</sup>N<sub>NO<sub>3</sub></sub> Plot Can Be Used to Identify a Typical Expected Isotopic Range of Denitrification for NO<sub>3</sub>-Impacted Groundwaters

2024· article· en· W4404965809 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS ES&T Water · 2024
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsCégep de ChicoutimiUniversity of CalgaryUniversité du Québec à ChicoutimiUniversity of Waterloo
FundersMinisterio de Ciencia, Innovación y Universidades
KeywordsPhysicsChemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Stable isotope values of δ 15 N NO 3 and δ 18 O NO 3 of dissolved nitrate (NO 3 ) are commonly used to identify the occurrence of denitrification as there is a progressive increase of δ 15 N NO 3 and δ 18 O NO 3 values accompanied by a decrease in NO 3 concentration. Thus, denitrification results in a positive trendline on the dual plot of δ 18 O NO 3 versus δ 15 N NO 3 . The combination of two trendlines with different slopes provides the “typical expected isotopic range of denitrification (TEIRD)” on the δ 18 O NO 3 versus δ 15 N NO 3 plot. Many studies distinguished denitrified groundwaters by applying the TEIRD concept that is incorrectly introduced because it assumes a single NO 3 source even though multiple NO 3 sources exist. Also, most TEIRD applications rely on specific denitrification slopes although these are known to vary owing to the aquifer’s changing biogeochemical conditions. Alternatively, an accurate delineation of the TEIRD requires the identification of all potential NO 3 sources in aquifer with their measured or reconstructed δ 15 N NO 3 and δ 18 O NO 3 values. This allows then for an accurate TEIRD to be traced with two denitrification trendlines having a slope corresponding to that from the correlation of the measured δ 18 O NO 3 and δ 15 N NO 3 values. Ultimately, each NO 3 source can have a specific TEIRD, although denitrification trendlines for multiple NO 3 sources can feature the same slope within a single aquifer.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0020.002
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0010.002
Science and technology studies0.0010.001
Scholarly communication0.0020.002
Open science0.0030.000
Research integrity0.0020.002
Insufficient payload (model declined to judge)0.0000.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.031
GPT teacher head0.242
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it