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Nanoscale Analyses of X-ray Amorphous Material from Terrestrial Ultramafic Soils Record Signatures of Environmental Conditions Useful for Interpreting Past Martian Conditions

2024· article· en· W4405053846 on OpenAlexaboutno aff
Anthony Feldman, Elisabeth M. Hausrath, E. B. Rampe, T. G. Sharp, Oliver Tschauner, Antonio Lanzirotti, M. Newville

Bibliographic record

VenueACS Earth and Space Chemistry · 2024
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPlanetary Science and Exploration
Canadian institutionsnot available
FundersUniversity of Nevada, Las VegasNevada Space Grant ConsortiumNational Aeronautics and Space Administration
KeywordsUltramafic rockMartianAstrobiologyAmorphous solidNanoscopic scaleSoil waterEarth scienceMars Exploration ProgramGeologyEnvironmental scienceMaterials scienceGeochemistrySoil sciencePhysicsChemistryNanotechnology

Abstract

fetched live from OpenAlex

The secondary mineral assemblage of martian rocks and sediments is critical to the interpretation of past conditions on Mars. X-ray amorphous material that is variably Mg/Fe/Si-rich and Al-poor, and that likely contains secondary alteration products, makes up between 15 and 73 wt % of Gale crater materials measured by the CheMin instrument and is also prevalent on the martian surface in other locations. Despite its prevalence, the structure and origin of this material and its implications for past martian environments remains unknown. Here, we employ transmission electron microscopy and synchrotron microprobe analyses of Fe/Si/Mg-rich and Al-poor ultramafic soils from the mediterranean climate Klamath Mountains of California and subarctic climate Tablelands of Newfoundland, Canada to help interpret environmental conditions during the formation of chemically similar X-ray amorphous material in Gale crater, Mars. X-ray amorphous material includes globular amorphous silica and chemically heterogeneous nanospherical amorphous material and nanocrystalline phases. Amorphous silica is present only in soils that undergo extensive periods of cyclic freezing conditions. X-ray amorphous material from the subarctic Tablelands is significantly richer in Mg and Si than material from the warmer Klamath Mountains. Nanocrystallites in both examined soils are richer in Fe than the truly amorphous material. However, Fe-rich nanocrystallites contain significantly more Mg and Si in the subarctic Tablelands, whereas Klamath Mountains soils contain highly Fe-enriched nanocrystallites incorporating little Mg and Si and potentially contain nanocrystalline smectites. These characteristics provide helpful identifiers to interpret past environmental conditions during the formation of X-ray amorphous material both in situ and in returned samples from Mars.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.459

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.238
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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