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Record W4405221188 · doi:10.1016/j.ces.2024.121051

Temperature impact on xanthate adsorption and microflotation of galena, sphalerite, and pyrite

2024· article· en· W4405221188 on OpenAlexafffund
D. S. Pashkevich, S. Mohammadi-Jam, Ozan Kökkılıç, Kristian E. Waters

Bibliographic record

VenueChemical Engineering Science · 2024
Typearticle
Languageen
FieldEnvironmental Science
TopicMinerals Flotation and Separation Techniques
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsXanthateSphaleriteGalenaPyriteAdsorptionChemistryInorganic chemistryEnvironmental chemistryMineralogyOrganic chemistry

Abstract

fetched live from OpenAlex

• Temperature effect on the flotation of galena, sphalerite and pyrite were investigated. • The microflotation yields corresponded well with the inverse gas chromatography surface energy results. • Adsorption kinetics of sodium isopropyl xanthate was heavily controlled by pH, temperature, and copper sulfate concentration. • Lower recovery of sphalerite at higher temperatures may be explained by the formation of calcium carbonate precipitates. • Lower recoveries at lower temperatures may be explained by a shift in the xanthate – oxy-complexes equilibrium. Selective flotation of lead–zinc ores is a process with many variables and a delicate balance of external (such as temperature) and internal factors (reagent concentrations, surface alterations). The purpose of this study is to explore flotation selectivity issues arising from changes in flotation pulp temperature. A deeper understanding of these issues can help to clarify industrial scale flotation discrepancies observed at different temperatures. Therefore, this paper provides insight into potential theoretical contributors to this balance, as well as assesses their affinity to temperature changes. These theoretical calculations assist in explaining observed variations in adsorption and microflotation results with temperature. Other statistically significant parameters influencing adsorption performance included xanthate concentration, copper sulfate dosage, and pH. Adsorption selectivity calculations were performed on individual mineral responses, which give insights into potential trends in the separation of galena, sphalerite, and pyrite. Adsorption results also confirmed current perceptions of the adsorption mechanism of dextrin. It has been shown that xanthate adsorption had the highest performance for galena among the three tested minerals. Scanning electron microscopy and EDS results allowed the extrapolation of a potential mechanism contributing to sphalerite depression at 45 °C. Inverse gas chromatography provided surface energy heterogeneity maps of the minerals. Surface energy values were generally in line with microflotation performance. The highest surface energy heterogeneity was observed for galena at 5 °C and for sphalerite at 45 °C. The role and variations in dissolved oxygen and lime dosages with temperature were also discussed with regard to flotation performance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.094
Threshold uncertainty score0.256

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.241
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2024
Admission routes2
Has abstractyes

Explore more

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