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An AOP-informed testing strategy to identify chemicals causing genotoxicity through oxidative DNA damage: case study on 4-nitroquinoline 1-oxide

2024· preprint· en· W4405430896 on OpenAlexaff
Elizabeth Huliganga, Eunnara Cho, Carol D. Swartz, Andrew Williams, Les Recio, Jesse J. Salk, Francesco Marchetti, Carole L. Yauk

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldBiochemistry, Genetics and Molecular Biology
Topicbioluminescence and chemiluminescence research
Canadian institutionsUniversity of OttawaHealth Canada
Fundersnot available
KeywordsGenotoxicityOxidative damageDNA damage4-Nitroquinoline 1-oxideChemistryDNAOxidative stressBusinessBiochemistryToxicityCarcinogenesisGene

Abstract

fetched live from OpenAlex

Adverse outcome pathways (AOPs) provide a framework to organize and weigh evidence linking molecular interactions of toxicants in cells to outcomes of regulatory concern. Applying this framework facilitates the interpretation of data produced using new test methods. We used AOP #296 which describes how oxidative DNA damage leads to mutations and chromosomal aberrations to develop an integrated testing strategy to evaluate whether a chemical operates through this pathway. We exposed human TK6 cells to increasing concentrations of 4-nitroquinoline 1-oxide (4NQO), a tobacco mimetic that causes oxidative DNA damage, in a time-series design. We measured oxidative DNA damage and strand breaks using the high-throughput CometChip assay with and without formamidopyrimidine DNA glycosylase (Fpg), alongside analyses of micronucleus (MN) frequency by flow cytometry, and mutations by error-corrected next-generation sequencing (Duplex Sequencing). Our analysis shows how these methods can be combined to quantify 4NQO-induced, concentration- and time-dependent increases in: (a) oxidative DNA damage (occurred early and at lower concentrations than single strand breaks); (b) strand breaks (remained elevated to 6 hours post-exposures); (c) MN frequency (at 24 hours); (d) mutation frequency (at 48 hours); and, (e) C>A transversions consistent with expected substitutions induced by oxidative DNA lesions. The time-series shows the repair of oxidative DNA damage with persistent strand breaks remaining at 6 hours. Overall, we provide an example of an AOP-informed testing strategy and contribute to quantitative understanding of AOP #296. We also demonstrate the high value of Duplex Sequencing for elucidating the mechanisms associated with exposure to oxidative stress inducers.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.019

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0040.004
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.096
GPT teacher head0.433
Teacher spread0.337 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2024
Admission routes1
Has abstractyes

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