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Record W4405431125 · doi:10.1139/cjc-2024-0150

Preparation of an adsorbent derived from canola hull by slow pyrolysis for effective carbon dioxide adsorption

2024· article· en· W4405431125 on OpenAlexafffundvenue
Qian Huang, Hari Karthik, Biswa R. Patra, Falguni Pattnaik

Bibliographic record

VenueCanadian Journal of Chemistry · 2024
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversity of Saskatchewan
FundersMitacs
KeywordsChemistryAdsorptionCanolaCarbon dioxidePyrolysisHullChemical engineeringOrganic chemistryComposite materialFood science

Abstract

fetched live from OpenAlex

Canola hull was proposed as a valuable precursor for activated carbon production, due to its abundance, low cost, and economic viability. This study aimed to develop a waste-based biosorbent from canola hulls by slow pyrolysis for effective CO2 capture. The biochar was synthesized from the canola hull using a fixed-bed tubular reactor through slow pyrolysis at various temperatures. The optimum biochar was activated using KOH as a chemical activating agent at different impregnation ratios. The biochar and activated carbon were characterized by elemental analysis, thermogravimetric analysis, surface textural analysis and FT-IR analysis. All the activated carbon samples with impregnation ratios of 0, 0.2, and 0.4 were screened at a total inlet mass flow rate of 100 mL/min (15% CO2 + 85% N2). Activated carbon prepared with an impregnation ratio of 0.4 (0.4AC) with a specific surface area of 1112 m2/g exhibited the highest adsorption capacity of CO2 (2.9 mmol/g) at 25 °C under ambient pressure when the feed gas was 15% CO2). 0.4AC was chosen for further study at different feed compositions. The breakthrough curves were analyzed for the compositions 5%, 15%, and 25% CO2 in feed, and the effects of adsorption parameters were discussed. The maximum CO2 uptake of the canola hull-based activated carbon (0.4AC) is 13.0 mmol/g at ambient pressure and 25 °C, with 100% CO2 inlet. Adsorption isotherm and kinetic were studied on the 0.4AC adsorbent. The canola hull-based adsorbent with desirable physiochemical and surface textural properties can work as an effective adsorbent for CO2 capture.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.208
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2024
Admission routes3
Has abstractyes

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